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Record W3200791844

Corrosion Inhibition of Piperazine for Potash Solution Mining and Processing Plants

2021· dissertation· en· W3200791844 on OpenAlexfundno aff
Ramasamy Thamilarasan

Bibliographic record

VenueoURspace (University of Regina) · 2021
Typedissertation
Languageen
FieldChemistry
TopicInorganic and Organometallic Chemistry
Canadian institutionsnot available
FundersUniversity of Regina
KeywordsPotashCorrosionPiperazineMetallurgyEnvironmental scienceEngineeringChemistryMaterials sciencePotassiumOrganic chemistry
DOInot available

Abstract

fetched live from OpenAlex

Potash mining and processing plants are prone to severe corrosion due to their operating conditions and potash brine constituents. Such corrosion causes a high expenditure on maintenance and repair of plant equipment and pipelines. To mitigate the corrosion, this work proposed the use of a corrosion inhibitor, namely piperazine (PZ) that is low toxic and commercially available. A series of electrochemical and weight loss corrosion experiments were carried out to examine corrosiveness of carbon steel (CS1018), J55 steel and stainless steel (SS316L) as well as to evaluate inhibition performance of PZ in saturated potash brines under the test conditions of 0 – 3880 rpm rotational speed, 25 – 85oC brine temperature and 1 – 5 bar pressure. Results show that CS1018 and J55 were much more corrosive than SS316L in saturated potash brine environments. Pitting tendency was observed on both CS1018 and J55. A higher rotational speed caused corrosion rates of CS1018 and J55 to increase. Increasing brine temperature caused CS1018 to be slightly less corrosive but caused J55 to become more corrosive. PZ was found to significantly reduce corrosion rate of CS1018 and J55 with the inhibition efficiency of 89.93 ± 0.87% and 87.20 ± 1.87% respectively, without pitting tendency at 85°C, 1 bar and 3880 rpm. Its high inhibition performance could be maintained over long durations (i.e. 21 and 28 days). PZ functioned as the mixed-type corrosion inhibitor retarding anodic and cathodic corrosion reactions. It protected the metal surface by undergoing monolayer chemisorption obeying the Langmuir adsorption isotherm on CS1018 and the Temkin adsorption isotherm on J55. The chemisorption was spontaneous and endothermic. PZ was likely to donate electrons to the metal surface during chemisorption. The presence of PZ did not alter purity and yield of potash products from a crystallization process.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.242
Threshold uncertainty score0.933

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.203
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2021
Admission routes1
Has abstractyes

Explore more

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