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A quantitative analysis of the ignition characteristics of fine iron particles

2022· article· en· W3209516027 on OpenAlexafffund
XiaoCheng Mi, Aki Fujinawa, Jeffrey M. Bergthorson

Bibliographic record

VenueCombustion and Flame · 2022
Typearticle
Languageen
FieldEngineering
TopicCombustion and Detonation Processes
Canadian institutionsMcGill University
FundersCanadian Space Agency
KeywordsIgnition systemMaterials scienceParticle sizeParticle (ecology)CombustionSuspension (topology)OxideDiffusionIron oxideThermodynamicsAnalytical Chemistry (journal)Radiative transferPhysicsChemistryOpticsPhysical chemistryMetallurgyChromatography

Abstract

fetched live from OpenAlex

Ignition of iron particles in an oxidizing environment marks the onset of self-sustained combustion. The objective of the current study is to quantitatively examine the ignition characteristics of fine iron particles (i.e., 1µm- to 100µm-sized) governed by the kinetics of solid-phase iron oxidation. The oxidation rates are inversely proportional to the thickness of the oxide layer (i.e., following a parabolic rate law) and calibrated using the experimentally measured growth of iron-oxide layers over time. Steady-state (i.e., Semenov’s analysis) and unsteady analysis have been performed to probe the dependence of the critical gas temperature required to trigger a thermal runaway (namely, the ignition temperature Tign) on particle size, initial thickness of oxide layer, inert gas species, radiative heat loss, and the collective heating effect in a suspension of particles. Both analyses indicate that Tign depends on δ0, i.e., the ratio between the initial oxide layer thickness and particle size, regardless of the absolute size of the particle. The unsteady analysis predicts that, for δ0≲0.003, Tign becomes independent of δ0. Under standard conditions in air, Tign is approximately 1080 K for any particle size greater than 5µm. The ignition temperature decreases as the thermal conductivity of the oxidizing gas decreases. Radiative heat loss has a minor effect on Tign. The collective effect of a suspension of iron particles in reducing Tign is demonstrated. The transition behavior between kinetic-controlled and external-diffusion-controlled combustion regimes of an ignited iron particle is systematically examined. The influences of initial oxide-layer thickness and particle temperature on the ignition delay time, τign, of iron particles are parametrically probed. A d2-law scaling between τign and particle size is identified. Possible sources of inaccuracy are discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.227
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations129
Published2022
Admission routes2
Has abstractyes

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