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Record W32508438 · doi:10.4103/jomfp.jomfp_149_20

The MoRe Isotopes Project: Production of high specific activity Mo-99 via isotope separation

2010· article· en· W32508438 on OpenAlexaff
Thomas J. Ruth, Suzanne E. Lapi, J.M. D’Auria, Keith Ladouceur

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldPhysics and Astronomy
TopicNuclear Physics and Applications
Canadian institutionsSimon Fraser UniversityTRIUMF
Fundersnot available
KeywordsIsotopeMolybdenumSeparator (oil production)Nuclear engineeringIon sourceIsotope separationNeutron sourceRadiochemistryChemistryIonNeutronProcess engineeringNuclear physicsPhysics

Abstract

fetched live from OpenAlex

1485 Objectives The MoRe project is developing a high power, off-line isotope separator capable of producing large quantities of Mo-99 at high specific activity from feedstock produced via 98Mo(n,γ) and/or 100Mo(γ,n) routes. Methods A high power ion source coupled to a high resolution dipole magnet will be used to generate beams of molybdenum ions and separate the respective isotopes with the aim of producing Mo-99 with specific activity greater than 1,000 Ci/g. The feedstock for the separator system will be low specific activity Mo-99 generated from thermal neutron capture on Mo-98 or photon induced neutron emission on Mo-100. This approach may allow the use of existing reactors to produce commercial quantities of Mo-99 while eliminating the need to use highly enriched uranium-235 (HEU) targets or incurring expense of converting facilities to use LEU targets. Results Preliminary proof of principle experiments have demonstrated the feasibility of generating intense Mo ion beams. Construction of an ion source test facility incorporating all of the elements of the separator system is underway with the expectation that sufficient beam current and ionization efficiency can be achieved in order to demonstrate the feasibility of using this device for producing commercial quality and quantities of Mo-99. Conclusions The proposed system will have several advantages compared to other proposed solutions: (1) the Mo-99 produced will fit directly into the existing commercial Tc-99m generator supply chain, (2) the elimination of HEU and LEU targets, (3) the system can be used to generate the required target material (Mo-98/Mo-100) during the separation process, (4) simplify production chemistry and (5) can be used in conjunction with a neutron or photon source to create a more robust distributed supply system, all at lower estimated cost than most of the proposed solutions to the medical isotope shortage crisis. Research Support Phases one of this research were supported by an NSERC I2I grant. The present work is supported by AAPS Inc

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.301
Threshold uncertainty score0.254

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.269
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2010
Admission routes1
Has abstractyes

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