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Record W37505232 · doi:10.1021/acsami.3c04820

Implementasi Tri Dharma Perguruan Tinggi dalam Mendukung Disiplin Nasional

2004· article· en· W37505232 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueACS Applied Materials & Interfaces · 2004
Typearticle
Languageen
FieldSocial Sciences
TopicEducational Curriculum and Learning Methods
Canadian institutionsnot available
FundersCanada First Research Excellence Fund
KeywordsPhysicsHumanitiesPhilosophy

Abstract

fetched live from OpenAlex

The hydrogen pump technique has been shown to be an effective method to measure the effective protonic conductivity of intermediate layers (ILs) that mimic the catalyst layers used in proton exchange membrane fuel cells and electrolyzers. It has been hypothesized, however, that the technique is limited to testing ILs that are inactive during the hydrogen reaction as proton transport through the ionomer in the layer can be bypassed by transferring the charge to the electronic phase via the reaction. This work uses numerical modeling, supported by experimental testing, to investigate the impact of IL hydrogen reaction activity, thickness, and electronic conductivity on the prediction of the IL protonic conductivity. A transient, 2-D, through-the-channel model is developed and implemented using the finite element method to predict the performance of hydrogen pump cells and perform electrochemical impedance spectroscopy. It is shown both numerically and experimentally that for iridium black and for platinum-/carbon-based ILs, the protonic phase is almost entirely bypassed, reducing the overall cell resistance and making the determination of the true conductivity difficult. The model can be used to provide an estimate of the resistance of the active layers, which is not possible using only experiments. In addition, the interfacial contact resistance between the membrane and the catalyst layers is determined using the high-frequency resistance, and the alternating current method for the hydrogen pump is studied to determine the accuracy of the method. Finally, further insights are provided through a breakdown of the resistances of each phase, as well as the potential profiles, in an active IL, and through parametric studies on the impact of varying the IL activity, thickness, and electronic conductivity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.129
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.037
GPT teacher head0.384
Teacher spread0.348 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it