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Record W4200292911 · doi:10.2138/am-2022-8309

Nanostructure reveals REE mineral crystallization mechanisms in granites from a heavy REE deposit, South China

2021· article· en· W4200292911 on OpenAlexaff
Aiguo Shi, Cheng Xu, Anton R. Chakhmouradian, Martin Smith, Jindřích Kynický, Chaoxi Fan, Chunwan Wei, Guangxi Kuang

Bibliographic record

VenueAmerican Mineralogist · 2021
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeochemistry and Elemental Analysis
Canadian institutionsUniversity of Manitoba
FundersNatural Environment Research CouncilSight Research UK
KeywordsGeochemistryHydrothermal circulationGeologyCrystallizationWeatheringQuartzMineralogyPetrographyMineralMineralization (soil science)Chemical engineeringMaterials scienceMetallurgy

Abstract

fetched live from OpenAlex

Abstract Weathering crusts after granites are the most important source of heavy rare-earth elements (HREE) worldwide. Although HREE in these deposits is known to be inherited from parental rocks, the origin of HREE enrichment and the reasons why it is rare outside of China remains unclear. Here, we report the occurrence of variably organized nanoparticles of Ce-poor (<0.2 wt%), Nd-Y-rich bastnäsite-(La), and associated cerianite in parental granites from a HREE deposit, South China. The mineral contains high-HREE abundances (up to 13 wt% Y2O3). Synchrotron radiation-induced X-ray diffraction and high-resolution transmission electron microscopy analyses suggest that the mineral grew as disordered nanocrystals and (nearly) coaligned nanoparticle aggregations, thus supporting “nonclassical” crystallization mechanisms by particle attachment under hydrothermal conditions. The nanocrystal-line Ce-poor, Nd-Y-rich bastnäsite-(La) precipitated at rapidly decreasing temperature related to the influx of externally derived fluids, which caused CO2-H2O immiscibility and REE supersaturation. This interpretation is supported by petrographic data and microthermometric analysis of fluid inclusions in quartz. Unusually high fO2 resulted in Ce oxidation and decoupling from trivalent lanthanides, producing polycrystalline mineralization.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.097
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.192
Teacher spread0.186 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2021
Admission routes1
Has abstractyes

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