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Record W4200554626 · doi:10.1029/2021je006992

Isotopic Composition of CO<sub>2</sub> in the Atmosphere of Mars: Fractionation by Diffusive Separation Observed by the ExoMars Trace Gas Orbiter

2021· article· en· W4200554626 on OpenAlexfundno aff
Juan Alday, Colin Wilson, P. G. J. Irwin, Аlexander Trokhimovskiy, Franck Montmessin, Anna Fedorova, Denis Belyaev, Kevin Olsen, Oleg Korablev, Franck Lefèvre, Ashwin Braude, Lucio Baggio, Andrey Patrakeev, Alexey Shakun

Bibliographic record

VenueJournal of Geophysical Research Planets · 2021
Typearticle
Languageen
FieldPhysics and Astronomy
TopicPlanetary Science and Exploration
Canadian institutionsnot available
FundersScience and Technology Facilities CouncilNatural Sciences and Engineering Research Council of CanadaMinistry of Education and Science of the Russian FederationCentre National d’Etudes SpatialesEuropean Space AgencyAgence Nationale de la RechercheUK Space Agency
KeywordsAtmosphere of MarsMars Exploration ProgramAtmosphere (unit)Trace gasIsotopologueAstrobiologyOrbiterFractionationMartian surfaceMartianAtmospheric escapeCarbonateAtmospheric chemistryAtmospheric sciencesGeologyEnvironmental scienceChemistryPhysicsMeteorologyAstronomy

Abstract

fetched live from OpenAlex

Abstract Isotopic ratios in atmospheric CO 2 are shaped by various processes throughout Mars' history, and can help understand what the atmosphere of early Mars was like to sustain liquid water on its surface. In this study, we monitor the O and C isotopic composition of CO 2 between 70 and 130 km for more than half a Martian year using solar occultation observations by the Atmospheric Chemistry Suite onboard the ExoMars Trace Gas Orbiter. We find the vertical trends of the isotopic ratios to be consistent with the expectations from diffusive separation above the homopause, with average values below this altitude being consistent with Earth‐like fractionation ( δ 13 C = −3 ± 37‰; δ 18 O = −29 ± 38‰; and δ 17 O = −11 ± 41‰). Using these measurements, we estimate that at least 20%–40% of primordial C on Mars has escaped to space throughout history. The total amount of C lost from the atmosphere is likely to be well in excess of this lower limit, due to carbonate formation and further sink processes. In addition, we propose a photochemical transfer of light O from H 2 O to CO 2 to explain the larger enrichment in the ratio in H 2 O than in CO 2 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.407
Threshold uncertainty score0.208

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.037
GPT teacher head0.316
Teacher spread0.279 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2021
Admission routes1
Has abstractyes

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