MétaCan
Menu
Back to cohort
Record W4205228019 · doi:10.1002/aoc.6612

Novel CoFe<sub>2</sub>O<sub>4</sub>/CuBi<sub>2</sub>O<sub>4</sub> heterojunction p–n semiconductor as visible‐light‐driven nanophotocatalyst for C (OH)–H bond activation

2022· article· en· W4205228019 on OpenAlex
Mahdieh Ghobadifard, Pavle V. Radovanovic, Sajjad Mohebbi

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueApplied Organometallic Chemistry · 2022
Typearticle
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of KurdistanUniversity of Waterloo
KeywordsHeterojunctionNanocompositePhotocatalysisChemistryVisible spectrumCharge carrierPhotochemistrySemiconductorNanostructureThermal stabilityNanoparticleReactivity (psychology)NanotechnologyMaterials scienceOptoelectronicsCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Nanosized CoFe 2 O 4 /CuBi 2 O 4 heterostructure was obtained by solvent‐free thermal processing and was characterized using a series of structural, physicochemical, and analytical techniques. The CuBi 2 O 4 and CoFe 2 O 4 nanoparticles demonstrated poor photoactivity due to their fast charge recombination and negligible visible light absorptivity, respectively. In contrast, the prepared heterojunction CoFe 2 O 4 /CuBi 2 O 4 nanocomposite consisting of an array of nanocolumns approximately 20 nm in width displayed nearly twofold higher photocatalytic activity than CoFe 2 O 4 or CuBi 2 O 4 nanostructures alone toward the C (OH)–H bond activation. This nanocomposite exhibits photocatalytic efficiency as high as 98% with very high stability. The increased photocatalytic reactivity could be related to the effective Z‐scheme mechanism of photogenerated charge carrier separation between CoFe 2 O 4 and CuBi 2 O 4 in the nanocomposite, which reduces the electron–hole recombination. The results of this work provide a promising approach to the design and preparation of heterostructured photocatalysts for oxidation reactions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Research integrity
Consensus categoriesMeta-epidemiology (narrow), Research integrity
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0030.003
Meta-epidemiology (broad)0.0030.001
Bibliometrics0.0010.004
Science and technology studies0.0020.001
Scholarly communication0.0000.001
Open science0.0020.002
Research integrity0.0010.003
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.225
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it