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Record W4210899179 · doi:10.1021/acs.jpcc.1c10577

TiO<sub>2</sub> Nanotubes: Morphology, Size, Crystallinity, and Phase-Dependent Properties from Synchrotron-Spectroscopy Studies

2022· article· en· W4210899179 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2022
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanada Foundation for Innovation
KeywordsAnataseMaterials scienceXANESRutileNucleationAmorphous solidAnnealing (glass)LuminescenceAnalytical Chemistry (journal)CrystallinityPhase transitionSpectroscopyChemical engineeringCrystallographyChemistryOptoelectronicsCondensed matter physicsPhotocatalysisMetallurgyComposite material

Abstract

fetched live from OpenAlex

This work presents a study of two series (anodization-time-dependent and anodization-voltage-dependent) of TiO2 nanotubes (NTs) prepared via control anodization and annealing methods. The desired phases of amorphous, anatase, mixed-phase (anatase and rutile), and rutile have been obtained, and their size-dependent phase transition behavior is investigated using synchrotron-based X-ray techniques. The local symmetry and electronic properties and the origin of luminescence from the TiO2 NTs are tracked by X-ray absorption near-edge structures (XANES) and X-ray excited optical luminescence (XEOL) techniques, respectively. It is found that the anatase-to-rutile (A-R) transition at a given annealing temperature highly depends on the size of NTs. That is, the longer the NTs, the slower the A-R phase transformation that would take place, while shorter NTs have a lower anatase fraction in the mixed-phase structure at the same annealing temperature. In addition, surface nucleation dominates the A-R phase transition in the temperature range of 700–800 °C. The power of XANES and XEOL in phase recognition is illustrated.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.593

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.259
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it