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Record W4220656562 · doi:10.5194/egusphere-egu22-11558

Nanoscale apatite inclusions in xenotime: witness of Pb mobility

2022· preprint· de· W4220656562 on OpenAlexaboutno aff
Cilva Joseph

Bibliographic record

Venuenot available
Typepreprint
Languagede
FieldBiochemistry, Genetics and Molecular Biology
TopicAdvanced Electron Microscopy Techniques and Applications
Canadian institutionsnot available
Fundersnot available
KeywordsAdenine nucleotideChemistryInternal medicineNucleotideBiochemistryMedicine

Abstract

fetched live from OpenAlex

Nanoscale apatite inclusions in xenotime: witness of Pb mobility Cilva Joseph1, 2, Denis Fougerouse1, 2, Steven M. Reddy1, 2, Aaron Dodd3, Steven Denyszyn4, David W. Saxey2, William D.A. Rickard2 1School of Earth and Planetary Sciences, Curtin University, Perth, Australia 2Geoscience Atom Probe Facility, John de Laeter Centre, Curtin University, Perth, Australia 3Microscopy and Microanalysis Facility, John De Laeter Centre, Curtin University, Perth, Australia 4School of Earth Sciences, University of Western Australia, Perth, Australia Discordant ages as measured by 206Pb/238U and 207Pb/235U ratios in various geochronometers are common. Several mechanisms have been proposed to explain discordant ages in different minerals. These include loss of radiogenic Pb, mixing of different age domains within a mineral, and intermediate daughter radioisotope disequilibrium. Xenotime (YPO4) is a geochronometer used to date different geological processes, such as diagenesis, metamorphism, and hydrothermal events. However, xenotime commonly yields small degrees of discordancy (<3%) by high precision geochronology techniques. To investigate the mechanism responsible for slightly discordant xenotime analyses, two ~1000 Ma crystals (z6413 and Y1) from Ontario and Western Australia were analysed using atom probe tomography (APT) and transmission electron microscopy (TEM) which provide sub-nanometre scale chemical and crystallographic analysis of minerals. Both samples have not undergone significant metamorphism (T < 300°C) after crystallisation. Combined APT and TEM results revealed the presence of nanoscale apatite [Ca5(PO4)3(F,Cl,OH)] inclusions and crystal dislocations in the xenotime grains. APT data indicates that the apatite inclusions are rich in radiogenic Pb and that the dislocations are decorated with Ca, Cl and H. Nanogeochronology of xenotime by APT indicate that the apatite inclusions likely formed by exsolution during the cooling of crystals, capturing radiogenic Pb. Dislocations in the crystals may have acted as fast diffusion pathways leading to radiogenic Pb-loss and caused the U-Pb system disturbance.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.020

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0060.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.322
Teacher spread0.315 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

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