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Record W4220863480 · doi:10.1021/acsapm.1c01671

Simulated Recycling of Polypropylene and Maleated Polypropylene for the Fabrication of Highly-Filled Wood Plastic Composites

2022· article· en· W4220863480 on OpenAlexafffund
Dylan Jubinville, Costas Tzoganakis, Tizazu H. Mekonnen

Bibliographic record

VenueACS Applied Polymer Materials · 2022
Typearticle
Languageen
FieldMaterials Science
TopicNatural Fiber Reinforced Composites
Canadian institutionsUniversity of Waterloo
FundersNatural Resources Canada
KeywordsPolypropyleneMaterials scienceWood flourMaleic anhydrideComposite materialComposite numberUltimate tensile strengthWood-plastic compositeIzod impact strength testMelt flow indexPolymerCopolymer

Abstract

fetched live from OpenAlex

In this study, polypropylene [PP] and maleic anhydride grafted polypropylene [MAPP] were reprocessed from one to three times to simulate recycling. 30 wt % of the reprocessed PP and MAPP were compounded with 70 wt % wood filler to fabricate highly filled wood plastic composites [WPCs]. The neat and composite samples were produced using a batch mixer and injection molder. The effect of recycling and maleation of PP was analyzed using light scattering, nuclear magnetic resonance, rheology, microscopy, and other physical/mechanical properties. While thermomechanical processing may lead to chain scission reactions, shown by a reduction in melt viscosity and weight-average molecular weight, the observed changes are minor and did not change the bulk properties significantly. The repeated reprocessing allowed for the incorporation of up to 70 wt % wood flour [WF] to fabricate the highly filled WPC while the maleation allowed for better interactions and the composite’s strength. Overall, the WPCs with maleic anhydride displayed appealing physical properties due to their increased tensile properties and a lack of oxidation or significant level of degradation. This indicates that the maleation of reprocessed PP could be an important and effective strategy to reduce virgin and petroleum-based MAPP while revitalizing mechanical properties for WPCs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.230
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations30
Published2022
Admission routes2
Has abstractyes

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