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Record W4223945796 · doi:10.5539/ijc.v14n1p23

Catalysis Mechanism and Application of Carbon Gasification Reaction-A Comparison of Two Heterogeneous Catalysis Mechanisms

2022· article· en· W4223945796 on OpenAlexvenueno aff
Jia Jin

Bibliographic record

VenueInternational Journal of Chemistry · 2022
Typearticle
Languageen
FieldMaterials Science
TopicHydrogen Storage and Materials
Canadian institutionsnot available
Fundersnot available
KeywordsCatalysisChemistryMechanism (biology)Catalytic cycleHeterogeneous catalysisReaction mechanismChemical engineeringComputational chemistryOrganic chemistryPhysicsQuantum mechanics

Abstract

fetched live from OpenAlex

This article is a brief summary article of research. The results of the three times experiments are reviewed. two heterogeneous catalysis mechanisms are introduced, namely: Chemical Reaction Mode Cyclic Catalysis Mechanism-CRM and Electron Cyclic Donate-Accept Catalysis Mechanism-ECDAM or Electron Orbital Deformation-Recovery Cyclic Catalysis Mechanism -EODRM. Some difficulties encountered by CRM are listed. The author clearly points out that the CRM is not credible. This false theory has misled us for more than 100 years. About ECDAM, the article also gives a brief description. The main point of ECDAM is that the catalysis phenomenon are physical rather than chemical phenomenon. The catalysts do not participate in chemical reactions. It's just contact, electron cyclic donate-accept or electron orbital deformation-recovery cycle. The theory contains three viewpoints: 1. There is a boundary between the catalyst and the poison. 2. The active of the catalyst or the degree of toxicity of the poison is closely related to the electronegative value of the catalyst or poison. 3. The active of catalyst is closely related to the chemical state of the catalyst The selectivity of catalyst is also related to electronegative or energy level According to ECDAM, the author considers that there are several problems worth studying in production and scientific research. such as: alumina is a poison in the Fe ammonia synthesis catalyst. The Cordierite (2MgO·2Al2O3·5SiO2) ceramic honeycomb support is also a poison in automotive exhaust purification catalyst. The Cordierite ceramic honeycomb is retardant in wall flow filter for diesel vehicles. Activated carbon is a poison in the Ruthenium catalyst for ammonia synthesis. Alumina and activated carbon all are a poison to noble metal catalysts, and so on.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.399

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.281
Teacher spread0.271 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

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