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Record W4225104223 · doi:10.3390/min12020171

Phosphate Removal from Wastewater by Magnetic Amorphous Lanthanum Silicate Alginate Hydrogel Beads

2022· article· en· W4225104223 on OpenAlexafffund
Hongyun Chen, Hongbo Zeng, Huaming Yang

Bibliographic record

VenueMinerals · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicPhosphorus and nutrient management
Canadian institutionsUniversity of Alberta
FundersNational Science Fund for Distinguished Young ScholarsChina Scholarship CouncilCentral South UniversityNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of ChinaCanada Research Chairs
KeywordsAdsorptionAqueous solutionPhosphateLanthanumAmorphous calcium phosphateAmorphous solidSilicateSodium silicateChemical engineeringInorganic chemistryMesoporous materialChemistryMaterials scienceNuclear chemistryOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

It is of both fundamental and practical importance to develop effective adsorbents for removing phosphate from aqueous solutions continuously. In this study, magnetic amorphous lanthanum silicate alginate hydrogel beads (MALS-B) were prepared and used for phosphate removal. Mesoporous silica materials with highly ordered and hexagonal channel structures were synthesized from natural mineral rectorite (REC) at room temperature. On this basis, amorphous lanthanum silicate (ALS) was synthesized by theone-pot method using a silicon source from REC and a commercial lanthanum source. Further, MALS-B were synthesized from sodium alginate (SA) with ALS and Fe3O4 as the incorporated adsorbable and magnetic nanoparticles via a simple cross-linking method in CaCl2 solution. The synthesized hydrogel beads were characterized by various techniques. ALS and Fe3O4 existed relatively independently in MALS-B, where ALS provided adsorption sites and Fe3O4 provided magnetism. They played a synergistic role in phosphate removal. The saturation magnetization value of MALS-B was 17.38 emu/g, enabling theirfacile separation from aqueous solutions after phosphate adsorption. MALS-B exhibited a preferable adsorption capacity of 40.14 mg P/g for phosphorus compared to other hydrogel beads based on adsorption experiments. More significantly, MALS-B exhibited excellent selectivity for phosphate in aqueous solutions with various interfering ions and possessed a high affinity to phosphate in a wide pH range. MALS-B showed the treatment volume of 480 BV when effluent phosphate concentration was below 0.5 mg/L in fixed-bed column adsorption. The adsorption mechanism was also revealed. Our work demonstrates that MALS-B can serve as a promising adsorbent for continuous phosphate adsorption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.186
Teacher spread0.180 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations21
Published2022
Admission routes2
Has abstractyes

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