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Supplementary material to "Biomass-burning derived particles from a wide variety of fuels: Part 1: Properties of primary particles"

2019· preprint· en· W4235771011 on OpenAlexaff
Crystal D. McClure, Christopher Y. Lim, David H. Hagan, Jesse H. Kroll, Christopher D. Cappa

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsSpectroscopyPhotoacoustic spectroscopyAnalytical Chemistry (journal)Integrating sphereAbsorption (acoustics)ChemistryAbsorption spectroscopyMaterials scienceLight scatteringMolar absorptivitySpectrometerPhotoacoustic imaging in biomedicineOpticsScatteringChromatographyPhysics

Abstract

fetched live from OpenAlex

Particle Optical Property MeasurementsParticle optical properties for PM1 were measured at 405 nm and 532 nm using the UC Davis Cavity Ringdown-Photoacoustic Spectrometer (CRD-PAS).In the UC Davis CRD-PAS, Light absorption coefficients (babs; units = Mm -1 ) for dry particles are determined using photoacoustic spectroscopy (Lack et al., 2012b).Light extinction coefficients (bext; units = Mm -1 ) for dry (<20% relative humidity) particles are measured at 405 nm and 532 nm via cavity ringdown spectroscopy (Langridge et al., 2011).Humidified light extinction measurements (RH ~85%) are also measured at 532 nm by cavity ringdown spectroscopy.The absorption measurements from the PAS were calibrated relative to the extinction measurement from the CRD using gas-phase O3 and NO2 with an estimated accuracy of 5% at 532 nm and 8% at 405 nm.Light absorption and scattering coefficients were also measured at 781 nm using a commercial PASS-3 photoacoustic spectrometer (DMT, Inc.).In the PASS-3, light absorption coefficients are measured by photoacoustic spectroscopy.Light scattering coefficients (bsca; units = Mm -1 ) are determined for dry particles with the PASS-3 using reciprocal nephelometry.The absorption measured by the

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.004
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Dataset · Consensus signal: Dataset
Teacher disagreement score0.646
Threshold uncertainty score0.505

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.004
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.002
Science and technology studies0.0010.000
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.6460.207

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.202
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

Study designNot applicable
Domainnot available
GenreDataset

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2019
Admission routes1
Has abstractyes

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