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Record W4243652375 · doi:10.1080/01418630050114745

Higher-order anharmonic contributions to the Debye-Waller factor

2000· article· en· W4243652375 on OpenAlexaff
Ramesh C. Shukla

Bibliographic record

VenuePhilosophical Magazine B · 2000
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAdvanced Chemical Physics Studies
Canadian institutionsBrock University
Fundersnot available
KeywordsAnharmonicityQuartic functionBravais latticeHamiltonian (control theory)Quintic functionBrillouin zonePhysicsHelmholtz free energyDebye–Waller factorMathematical physicsDiagrammatic reasoningQuantum mechanicsMathematicsChemistryCrystallographyCrystal structurePure mathematics

Abstract

fetched live from OpenAlex

We have presented a detailed analysis of the higher-order anharmonic contributions to the average square atomie displacement (u 2) or Debye-Waller factor by the diagrammatic method and the Zubarev type Green's function method. The Hamiltonian employed in the detailed analysis contains the anharmonic terms up to O(λ4)that is the cubic, quartic, quintic and sextic terms which arise from the Taylor expansion of the potential energy. Thus the various contributions to (u 2) of O(λ2) and O(λ4), presented in the diagrammatic language, arise from the first-, second-, third- and the fourth-order perturbation theory. This analysis establishing interrelationships between the Helmholtz free energy (F), self-energy and (u 2) reveals that a total of 16 diagrams contribute to (u 2) for a Bravais lattice or a lattice with a basis where every atom is at a site of inversion symmetry. A simple prescription is given for the derivation of (u 2) diagrams from the F diagrams. Out of 16 diagrams, two are of O(λ2) and 14 of O(λ4), where λ is a perturbation expansion parameter. It is also shown that at least up to O(λ4) the contributions to (u 2) from nine out of 16 diagrams are included in the Green's function iterative solution if the latter is generated from the anharmonic Hamiltonian containing the cubic and auartic terms. Exact and approximate numerical magnitudes for all the diagrams are obtained for a nearest-neighbour 6-12 Lennard-Jones fec solid by extrapolating the Brillouin zone (BZ) sums to the q → 0 limit. A disproportionate contribution to the BZ sums comes from this region of q space in the calculation of (u 2) In the context of (u 2) the importance of the various self-energy diagrams involving the same type of anharmonic vertices is established. It is shown that there exists a heavy cancellation among these 14 diagrams; nevertheless their total contribution to (u 2) is sufficient to bring it in almost exact agreement with the classical Monte Carlo results, which are also obtained for the same model.

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How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.032

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0100.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.287
Teacher spread0.269 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations0
Published2000
Admission routes1
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