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Record W4252654332 · doi:10.2174/2211334710801020093

Scrubber Designs for Enzyme-Mediated Capture of CO2

2008· article· en· W4252654332 on OpenAlexaff
Olivier Lacroix, Faı̈çal Larachi

Bibliographic record

VenueRecent Patents on Chemical Engineering · 2008
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicEnzyme function and inhibition
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsScrubberChemistryCarbonic anhydraseCarbon dioxideCarbonationBicarbonateCarbon dioxide removalChemical engineeringWaste managementEnvironmental chemistryOrganic chemistryEnzyme

Abstract

fetched live from OpenAlex

Carbon dioxide is the most abundantly emitted greenhouse gas for which several technologies are being developed and intensively studied for capture and storage, except retrofit of amine scrubbers, none is proven at the commercial scale for treating post-combustion stack gases. Amine scrubbing, membrane separation, wet and dry mineral carbonation, pressure, temperature and electrical swing adsorptions, have been thoroughly reviewed in the 2005 survey by the Intergovernmental Panel on Climate Change (IPCC). However, an innovative approach that has escaped the attention of the recent IPCC concerns using biocatalysts for carbon dioxide hydration to bicarbonate. This review critically evaluates the recent patent literature regarding the different scrubber configurations in use for supporting carbonic anhydrase (CA), an ultrafast zinc-bearing metalloenzyme which catalyzes CO2 hydration to bicarbonate. It describes two membrane contactors using free soluble CA, the first one releasing gaseous CO2 and the second one being used to produce precipitated calcium carbonate (PCC). It also describes two contactors using immobilized CA, namely counter-current and cross-co-current packed columns, and two other contactors using either free or particle-immobilized CA. The review also deals with the use of a cohort of enzymes mimicking metabolic pathways to capture CO2 and potentially produce useful organic compounds. Keywords: Carbon dioxide, capture, storage, recycling, enzymes, carbonic anhydrase, rubisco

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.029
GPT teacher head0.227
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2008
Admission routes1
Has abstractyes

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