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Comparative analysis of the structure of water-soluble LCCs and the Björkman LCCs in poplar wood

2022· preprint· en· W4280635925 on OpenAlexaff
Sheng Cui, Xin Wei, Xundong Chen

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldEngineering
TopicLignin and Wood Chemistry
Canadian institutionsUniversity of Alberta
FundersNational Natural Science Foundation of China
KeywordsLigninChemistryChemical structureEtherChemical compositionOrganic chemistry

Abstract

fetched live from OpenAlex

The structural study of lignin-carbohydrate complexes (LCCs) provides a theoretical basis for the high-value utilization of biomass which has always been a hot topic in biomaterials and biomass refining. This paper compares the structure of two types of LCCs in poplar. After poplar wood was crushed by ball milling, water-soluble LCCs and the Björkman LCCs were extracted by hot water extraction and the Björkman classical method, respectively. The molecular weight was determined by GPC, the composition was determined by chemical analysis, and the structure was studied by UV, IR and 2D-NMR. Comparing the two, the results showed that water-soluble LCCs contains a higher content of carbohydrates and has a relatively wide molecular weight distribution, while the carbohydrate content of the Björkman LCCs was relatively low, and the molecular weight distribution range was relatively narrow. UV, IR and 2D-NMR results confirmed that the main chemical links between the lignin units of the two LCCs were β-O-4. β-β, β-5 structures. The chemical linkages between lignin and carbohydrates in water-soluble LCCs were mainly phenyl glycosidic bonds and ester bonds, while in the Björkman LCCs, there were not only have phenyl glycosides bonds and ester bonds, but also found existence of ether bonds between lignin and carbohydrates. This work contributes to a comprehensive understanding of the structure of poplar LCCs and provides theoretical support for the further application of poplar wood.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.218
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations0
Published2022
Admission routes1
Has abstractyes

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