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Record W4281760522 · doi:10.3390/s22114175

A Wavelength Modulation Spectroscopy-Based Methane Flux Sensor for Quantification of Venting Sources at Oil and Gas Sites

2022· article· en· W4281760522 on OpenAlexafffund
Simon A. Festa-Bianchet, Scott P. Seymour, David R. Tyner, Matthew R. Johnson

Bibliographic record

VenueSensors · 2022
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsCarleton University
FundersNatural Resources CanadaNatural Sciences and Engineering Research Council of CanadaMitacs
KeywordsMethaneAllan varianceOpticsLaserMaterials scienceMulti-mode optical fiberVolume (thermodynamics)Absorption (acoustics)WavelengthStandard deviationAnalytical Chemistry (journal)Optical fiberOptoelectronicsChemistryPhysics

Abstract

fetched live from OpenAlex

An optical sensor employing tunable diode laser absorption spectroscopy with wavelength modulation and 2f harmonic detection was designed, prototyped, and tested for applications in quantifying methane emissions from vent sources in the oil and gas sector. The methane absorption line at 6026.23 cm−1 (1659.41 nm) was used to measure both flow velocity and methane volume fraction, enabling direct measurement of the methane emission rate. Two configurations of the sensor were designed, tested, and compared; the first used a fully fiber-coupled cell with multimode fibers to re-collimate the laser beams, while the second used directly irradiated photodetectors protected by Zener barriers. Importantly, both configurations were designed to enable measurements within regulated Class I / Zone 0 hazardous locations, in which explosive gases are expected during normal operations. Controlled flows with methane volume fractions of 0 to 100% and a velocity range of 0 to 4 m/s were used to characterize sensor performance at a 1 Hz sampling rate. The measurement error in the methane volume fraction was less than 10,000 ppm (1%) across the studied range for both configurations. The short-term velocity measurement error with pure methane was <0.3 m/s with a standard deviation of 0.14 m/s for the fiber-coupled configuration and <0.15 m/s with a standard deviation of 0.07 m/s for the directly irradiated detector configuration. However, modal noise in the multimode fibers of the first configuration contributed to an unstable performance that was highly sensitive to mechanical disturbances. The second configuration showed good potential for an industrial sensor, successfully quantifying methane flow rates up to 11 kg/h within ±2.1 kg/h at 95% confidence over a range of methane fractions from 25−100%, and as low as ±0.85 kg/h in scenarios where the source methane fraction is initially unknown within this range and otherwise invariant.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.250
Threshold uncertainty score0.576

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.272
Teacher spread0.251 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2022
Admission routes2
Has abstractyes

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