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Record W4281888213 · doi:10.1002/jsde.12597

Foaming and defoaming properties of <scp>CO<sub>2</sub></scp>‐switchable surfactants

2022· article· en· W4281888213 on OpenAlexafffund
Hailey Poole, Philip G. Jessop, Cosima Stubenrauch

Bibliographic record

VenueJournal of Surfactants and Detergents · 2022
Typearticle
Languageen
FieldChemistry
TopicSurfactants and Colloidal Systems
Canadian institutionsQueen's University
FundersNatural Sciences and Engineering Research Council of CanadaDeutscher Akademischer Austauschdienst
KeywordsPulmonary surfactantChemistryCationic polymerizationChemical engineeringBromideVolume (thermodynamics)MoleculeFoaming agentAmphiphileProtonationPolymer chemistryPorosityOrganic chemistryPolymerIonThermodynamicsCopolymer

Abstract

fetched live from OpenAlex

Abstract The present study is about the foaming and defoaming properties of the CO 2 ‐switchable surfactant N,N‐dimethyltetradecylamine (C 14 DMA) and its advantages compared with the non‐switchable counterpart tetradecyltrimethylammonium bromide (C 14 TAB). In the absence of CO 2 , C 14 DMA is a water insoluble organic molecule without any surface activity thus being unable to stabilize foams. In the presence of CO 2 , the head group becomes protonated which transforms the water insoluble molecule into a cationic surfactant. Comparing the surface properties and foamability of C 14 DMA and C 14 TAB one finds a very similar behavior. However, the foam stabilities differ depending on the gas. Foaming the two‐surfactant solutions with CO 2 leads to very unstable foams in both cases. However, foaming the two surfactant solutions with N 2 reveals the switchability of C 14 DMA: while the volume of foams stabilized with C 14 TAB hardly changes over 1600 s, the volume of foams stabilized with C 14 DMA decreases significantly in the same period of time. This difference is due to the fact that the surface activity, that is, the amphiphilic nature, of C 14 DMA is continuously switching off since CO 2 is displaced by N 2 thus deprotonating and deactivating the surfactant.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.142
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.211
Teacher spread0.192 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2022
Admission routes2
Has abstractyes

Explore more

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