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Record W4282599182 · doi:10.1021/acs.estlett.2c00311

Ozonolysis Lifetime of Tetrahydrocannabinol in Thirdhand Cannabis Smoke

2022· article· en· W4282599182 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnvironmental Science & Technology Letters · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicIndoor Air Quality and Microbial Exposure
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaAlfred P. Sloan Foundation
KeywordsThird-hand smokeSmokeOzoneContaminationEnvironmental chemistryOzonolysisChemistryCannabisDronabinolFraction (chemistry)Environmental scienceChromatographySidestream smokeOrganic chemistryMedicineCannabinoid

Abstract

fetched live from OpenAlex

Thirdhand smoke (THS) describes the persistent contamination on indoor surfaces following smoking. Cannabis THS is a chemically distinct form of THS which remains poorly characterized, relative to tobacco. Understanding its fate is necessary to mitigate exposure to cannabis smoke components and potentially harmful transformation products. In this work, the heterogeneous reaction of surface-bound Δ9-tetrahydrocannabinol (THC), a component of cannabis smoke, with ozone was examined. Cannabis smoke deposits were collected inside a Teflon chamber on glass, cotton, and tile surfaces. Samples were exposed to high (100 ppb) and realistic indoor ozone concentrations (20 ppb) inside a flow tube and to low ozone levels (2 to 29 ppb) present in a genuine indoor environment. Chemical transformations were monitored by liquid chromatography-tandem mass spectrometry (LC-MS/MS), with epoxide and dicarbonyl products detected. Rapid initial loss of THC was observed on all surfaces, but a small fraction (5%–10%) persisted for extended time scales. A short loss lifetime (a few hours) was observed for THC deposited on glass and tile under typical indoor ozone exposures, leading to almost complete loss at longer times. THC decay on cotton was approximately five times longer than on glass, with up to 10% of THC remaining after 1 week of exposure.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies, Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.191
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.002
Science and technology studies0.0010.004
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.196
Teacher spread0.192 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it