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Record W4283716908 · doi:10.1021/acs.iecr.2c01198

Graphene-Embedded Hybrid Network Structure to Render Olefin Block Copolymer Foams with High Compression Performance

2022· article· en· W4283716908 on OpenAlexaff
Yanting Li, Yunjie Liu, Pengjian Gong, Yanhua Niu, Chul B. Park, Guangxian Li

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2022
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Foaming and Composites
Canadian institutionsUniversity of Toronto
FundersState Key Laboratory of Polymer Materials EngineeringSichuan UniversityNational Natural Science Foundation of China
KeywordsGrapheneMaterials scienceLow-density polyethyleneCopolymerExfoliation jointNanocompositeChemical engineeringNucleationComposite materialPolymerPolymer chemistryNanotechnologyChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Graphene has abundant interactions with polymers by adhering to macromolecular chain segments, facilitating heterogeneous crystal nucleation and adsorbing free radicals. Hence, a hierarchical network structure using graphene as the anchor could be formed in an olefin block copolymer (OBC)/low-density polyethylene (LDPE) blend together with cross-linking points and entanglement points. Then, a nanocomposite foam was fabricated by supercritical CO2 foaming. In this work, a graphene-embedded hybrid network structure was designed to effectively control OBC/LDPE foaming. The strategy is as follows: (1) Macromolecular free radicals triggered by peroxide were adsorbed on the surface of graphene to form a dentritic-on-plate structure. (2) Both OBC and LDPE molecular chain segments were adhered to graphene to form a hybrid physical network. (3) Long-branched chains of LDPE formed entanglement points with both molecular chains whose segments adhered to graphene and macromolecular free radicals adsorbed on graphene. Finally, an optimized graphene content of 0.5 wt % in the obtained nanocomposite foam would maximize its compression stability (hysteresis loss of 53%) with a high resilience of 60%.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.166
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.029
GPT teacher head0.262
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations16
Published2022
Admission routes1
Has abstractyes

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