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Record W4283834209 · doi:10.1021/acsomega.2c02163

Antidiabetic and Cytotoxic Activities of Rotenoids and Isoflavonoids Isolated from <i>Millettia pachycarpa</i> Benth

2022· article· en· W4283834209 on OpenAlexaff
Virayu Suthiphasilp, Narawadee Rujanapun, Pakit Kumboonma, Boonyanoot Chaiyosang, Sarawut Tontapha, Tharakorn Maneerat, Brian O. Patrick, Raymond J. Andersen, Thidarat Duangyod, Rawiwan Charoensup, Surat Laphookhieo

Bibliographic record

VenueACS Omega · 2022
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicBioactive natural compounds
Canadian institutionsUniversity of British Columbia
FundersThailand Science Research and InnovationMae Fah Luang University
KeywordsPhytochemicalCytotoxicityChemistryCircular dichroismIC50StereochemistryTraditional medicineIn vitroBiochemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide A phytochemical investigation of the root and leaf extracts of Millettia pachycarpa Benth resulted in the isolation and identification of 16 compounds, including six rotenoids ( 1 – 6 ) and 10 prenylated isoflavonoids ( 7 – 16 ). Compound 4 was isolated as a scalemic mixture, which was resolved by chiral HPLC to afford (−)-(6a S,12a S )-12a-hydroxy-α-toxicarol ( 4 ) and (+)–(6a R,12a R )-12a-hydroxy-α-toxicarol ( 4 ). (+)-(6a R,12a R )-Millettiapachycarpin ( 3 ) and (−)-(6a S,12a S )-12a-hydroxy-α-toxicarol ( 4 ) were isolated as new compounds. The absolute configuration of (−)-(6 R )-pachycarotenoid ( 2 ), (+)–(6a R,12a R )-millettiapachycarpin ( 3 ), (−)-(6a S,12a S )- 4 and (+)–(6a R,12a R )-12a-hydroxy-α-toxicarol ( 4 ), (+)-(6a S,12a S )-( 5 ), and (−)-(6a S,12a S,2″ R )-sumatrol ( 6 ) were identified by electronic circular dichroism (ECD) data. (−)-(6a S,12a S,2″ R )-Sumatrol ( 6 ) was also confirmed by X-ray diffraction analysis using Cu–Kα radiation. Antidiabetic activities, including α-glucosidase and α-amylase inhibitory activities, and cytotoxicities against lung cancer A549, colorectal cancer SW480, and leukemic K562 cells of some isolated compounds were evaluated. Of these, isolupalbigenin ( 11 ) exhibited the highest α-glucosidase inhibitory activity, with an IC 50 value of 11.3 ± 0.2 μM, whereas the scalemic mixture of 12a-hydroxy-α-toxicarol ( 4 ) displayed the best α-amylase inhibitory activity, with an IC 50 value of 106.9 ± 0.2 μM. Euchrenone b10 ( 15 ) exhibited the highest cytotoxicity against lung cancer A549, colorectal cancer SW480, and leukemic K562 cells, with IC 50 values of 40.3, 39.1, and 15.1 μM, respectively. In addition, molecular docking simulations of α-glucosidase inhibition of the active compounds were studied.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.204
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations16
Published2022
Admission routes1
Has abstractyes

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