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Record W4285589444 · doi:10.1002/cjce.24550

Metal–organic frameworks‐derived <scp> TiO <sub>2</sub> </scp> for photocatalytic degradation of tetracycline hydrochloride

2022· article· en· W4285589444 on OpenAlexvenueno aff
Xin Wan, Guanglai Mo, Jianhong Luo

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2022
Typearticle
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsnot available
Fundersnot available
KeywordsPhotocatalysisMaterials scienceCalcinationChemical engineeringDegradation (telecommunications)Tetracycline HydrochlorideMetalTitaniumSpecific surface areaNanotechnologyCatalysisOrganic chemistryMetallurgyTetracyclineChemistryComputer science

Abstract

fetched live from OpenAlex

Abstract This work will change the common understanding that C doping of MIL‐125(Ti)‐derived TiO 2 is a key factor in improving its photocatalytic performance, and it can also help to understand the internal relationship between the structure and performance of photocatalytic materials deeply. It provides a simple synthesis method for the wider application of TiO 2 in the field of photocatalysis. Compared with previous studies, this article uses the titanium‐based metal‐organic framework MIL‐125(Ti) to prepare the semiconductor photocatalyst M‐TiO 2 by calcination in the air at a lower temperature and shorter time. After analyzing the M‐TiO 2 prepared in the experiment, the results can be received that there is no obvious agglomeration and the morphology is almost unchanged, as the frame structure does not collapse at the same time. As a result, the advantages of the large specific surface area and porousness of metal–organic frameworks (MOF) as precursor derivatives are preserved. As for the changes in the micro‐morphology, pore structure, and specific surface area of M‐TiO 2 compared with the precursor, they are investigated seriatim. The results show that, compared with commercial TiO 2 ‐P25, the performance of M‐TiO 2 photocatalytic degradation of tetracycline hydrochloride is 5.7 times that of the precursor metal‐organic framework MIL‐125(Ti) and 2.2 times that of P25, and has good cycle stability.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.198
Teacher spread0.188 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2022
Admission routes1
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical EngineeringSame topicMetal-Organic Frameworks: Synthesis and ApplicationsFrench-language works237,207