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Record W4290667764 · doi:10.1029/2022wr032182

Causes and Factors of Cryogenic Extraction Biases on Isotopes of Xylem Water

2022· article· en· W4290667764 on OpenAlexaff
Mingyi Wen, Dong He, Min Li, Ruiqi Ren, Jingjing Jin, Bingcheng Si

Bibliographic record

VenueWater Resources Research · 2022
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsUniversity of Saskatchewan
FundersNational Natural Science Foundation of China
KeywordsXylemDeuteriumExtraction (chemistry)IsotopeWater extractionStable isotope ratioEnvironmental chemistryEnvironmental scienceChemistryHydrogenBotanyBiologyChromatographyPhysicsNuclear physics

Abstract

fetched live from OpenAlex

Abstract Cryogenic vacuum extraction (CVE) has been considered as the standard technique for the analysis of plant water stable isotopes in ecohydrological research. Recent studies reported that CVE can introduce significant bias in stable isotope analyses, yet the causes and influencing factors of the CVE‐induced deuterium offsets remain poorly understood. Here, we performed rehydration experiments on plant samples from two species and three organs with two distinct‐isotopic spiking waters. Centrifugation and high‐pressure mechanical squeezing were used to separate sap water and tissue water for stable isotope analyses. Plant waters extracted by CVE differed significantly from reference waters in δ 2 H, but not in δ 18 O. The δ 2 H bias was linearly correlated to the xylem water content, and this relationship is affected significantly by plant organs/species and the isotopic signature of the spiking water. Moreover, the δ 2 H bias induced by CVE (−8.52 ± 0.90‰) was significantly greater than the δ 2 H difference between the tissue and sap waters (−3.33 ± 0.76‰) for apple stems possessing similar water contents. Thus, hydrogen‐exchange between plant organics and water, and isotopic heterogeneity within plants both contribute to the negative δ 2 H bias, but the former is the dominant cause. The multiple factors governing the CVE‐induced δ 2 H bias, make it difficult to establish a unified bias correction equation. Our results question the usefulness of cryogenic extraction as a standard for plant water extraction.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.553
Threshold uncertainty score0.994

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0070.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.071
GPT teacher head0.300
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations41
Published2022
Admission routes1
Has abstractyes

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