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Record W4292212875 · doi:10.2166/wpt.2022.095

Comparative efficiency of oxidation processes to remove acesulfame in water treatment plants supplied by surface water sources

2022· article· en· W4292212875 on OpenAlex
Jean Sérodes, Antoine Grondin, Sabrina Simard, Geneviève Pelletier, Manuel J. Rodríguez

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueWater Practice & Technology · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicWater Treatment and Disinfection
Canadian institutionsUniversité Laval
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsWater treatmentChlorineEnvironmental chemistryChemistryRaw waterOzoneWater qualitySurface waterOxidizing agentFlocculationEnvironmental scienceEnvironmental engineeringPulp and paper industryEcology

Abstract

fetched live from OpenAlex

Abstract The effects of oxidizing agents during water treatment on the concentration of an artificial sweetener were evaluated in full-scale conditions. Five drinking water treatment plants (DWTPs) located in a northern environment with high seasonal variations which use different raw water sources and different combinations of oxidants (ozone, chlorine, UV radiation) were investigated through the removal of the artificial sweetener acesulfame (ACE) along their treatment chains. In total, 98 sampling campaigns were conducted at these DWTPs. Raw water (impacted by variable tidal and hydrodynamic conditions), partially treated water within the DWTPs, and fully treated drinking water were sampled during eight months over the period of higher variability of source water quality. Results showed ACE concentrations in raw waters vary on a seasonal basis: higher in winter and summer (when rivers have low water discharges) and lower during spring and fall. Multi-barrier treatment systems under study were effective for the removal of acesulfame due specifically to the effect of ozone and chlorine during oxidation steps, while no removal was observed using physico-chemical (coagulation flocculation, filtration) and UV treatments. Depending on the number of treatment steps that involved ozonation or chlorination and the position of these oxidative processes in the treatment chain, removal of ACE varied from 24% to 90% in the plants under study. The results indicate that increasing oxidant doses would result in better removal of ACE and other contaminants, but these strategies must consider unknown transformation products, potentially with greater toxicological effects than their precursors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.043
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.248
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it