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Record W4297585557 · doi:10.1021/acsaenm.2c00001

Electrochemical Grafting of an Aminated Poly(methyl methacrylate) (PMMA)-like Liner onto a Silicon Surface for the Metallization of Microfeatures

2022· article· en· W4297585557 on OpenAlex
Gul Zeb, Xuan Tuan Le

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Applied Engineering Materials · 2022
Typearticle
Languageen
FieldEngineering
TopicMolecular Junctions and Nanostructures
Canadian institutionsCMC Microsystems (Canada)
Fundersnot available
KeywordsPassivationMaterials scienceAminationMethyl methacrylateChemical engineeringSiliconElectrochemistryPolymerLayer (electronics)Poly(methyl methacrylate)Deposition (geology)Aqueous solutionElectrolytePolymer chemistryPolymerizationNanotechnologyElectrodeComposite materialOrganic chemistryChemistryOptoelectronicsCatalysis

Abstract

fetched live from OpenAlex

The micro/nanofabrication industry’s transition from physically deposited dielectric films toward relatively inexpensive insulating polymeric materials faces a challenging metallization step in progression. In this work, we demonstrate a metallization scheme constituting simple and completely aqueous chemical steps─from Si passivation to metallization. We first propose a versatile diazonium-based electrochemical process to graft an in situ aminated poly(methyl methacrylate) (PMMA) liner onto Si microfeatures with high step-coverage. These amine-terminated groups functionalize the grafted PMMA-like liner with palladium chloride complex activators and allow direct autocatalytic deposition of Ni–B film while avoiding any further amination step as conventionally required for polymeric surfaces. The obtained Ni–B film exhibiting high uniformity, strong adhesion to the polymer film, and excellent step-coverage from the top, sidewall, and bottom of the microstructures fulfills all requirements of a conducting seed layer for the subsequent electrolytic deposition of copper.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.155
Threshold uncertainty score0.744

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.196
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it