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Record W4298151151 · doi:10.1002/advs.202105063

In‐MOF‐Derived Hierarchically Hollow Carbon Nanostraws for Advanced Zinc‐Iodine Batteries

2022· article· en· W4298151151 on OpenAlexaff
Lulu Chai, Xian Wang, Yue Hu, Xifei Li, Shaoming Huang, Junqing Pan, Jinjie Qian, Xueliang Sun

Bibliographic record

VenueAdvanced Science · 2022
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsWestern University
FundersFundamental Research Funds for the Central UniversitiesNational Key Research and Development Program of ChinaNational Natural Science Foundation of China
KeywordsZincMaterials scienceIodineCarbon fibersNanotechnologyChemical engineeringMetallurgyEngineeringComposite materialComposite number

Abstract

fetched live from OpenAlex

Abstract Hollow carbon materials are regarded as crucial support materials in catalysis and electrochemical energy storage on account of their unique porous structure and electrical properties. Herein, an indium‐based organic framework of InOF‐1 can be thermally carbonized under inert argon to form indium particles through the redox reaction between nanosized indium oxide and carbon matrix. In particular, a type of porous hollow carbon nanostraw (HCNS) is in situ obtained by combining the fusion and removal of indium within the decarboxylation process. The as‐synthesized HCNS, which possesses more charge active sites, short and quick electron, and ion transport pathways, has become an excellent carrier for electrochemically active species such as iodine with its unique internal cavity and interconnected porous structure on the tube wall. Furthermore, the assembled zinc‐iodine batteries (ZIBs) provide a high capacity of 234.1 mAh g−1 at 1 A g−1, which ensures that the adsorption and dissolution of iodine species in the electrolyte reach a rapid equilibrium. The rate and cycle performance of the HCNS‐based ZIBs are greatly improved, thereby exhibiting an excellent capacity retention rate. It shows a better electrochemical exchange capacity than typical unidirectional carbon nanotubes, making HCNS an ideal cathode material for a new generation of high‐performance batteries.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.271
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations139
Published2022
Admission routes1
Has abstractyes

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