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Record W4308144453 · doi:10.1088/2058-8585/ac9f54

Shellac-paper composite as a green substrate for printed electronics

2022· article· en· W4308144453 on OpenAlex
Rahaf Nafez Hussein, Kory Schlingman, Calum Noade, R. Stephen Carmichael, Tricia Breen Carmichael

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueFlexible and Printed Electronics · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicMicroplastics and Plastic Pollution
Canadian institutionsUniversity of Windsor
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsShellacMaterials sciencePolyethylene terephthalateElectronicsPolyethyleneDurabilityPrinted electronicsNanotechnologyInkwellCoatingComposite materialEngineeringElectrical engineering

Abstract

fetched live from OpenAlex

Abstract Printed electronic (PE) devices that sense and communicate data will become ubiquitous as the Internet of things continues to grow. Devices that are low cost and disposable will revolutionize areas such as smart packaging, but a major challenge in this field is the reliance on plastic substrates such as polyethylene terephthalate. Plastics discarded in landfills degrade to form micro- and nanoplastics that are hazardous to humans, animals, and aquatic systems. Replacing plastics with paper substrates is a greener approach due to the biodegradability, recyclability, low cost, and compatibility with roll-to-roll printing. However, the porous microstructure of paper promotes the wicking of functional inks, which adversely affects printability and electrical performance. Furthermore, truly sustainable PE must support the separation of electronic materials, particularly metallic inks, from the paper substrate at the end of life. This important step is necessary to avoid contamination of recycled paper and/or waste streams and enable the recovery of electronic materials. Here, we describe the use of shellac—a green and sustainable material—as a multifunctional component of green, paper-based PE. Shellac is a cost-effective biopolymer widely used as a protective coating due to its beneficial properties (hardness, UV resistance, and high moisture- and gas-barrier properties); nonetheless, shellac has not been significantly explored in PE. We show that shellac has great potential in green PE by using it to coat paper substrates to create planarized, printable surfaces. At the end of life, shellac acts as a sacrificial layer. Immersing the printed device in methanol dissolves the shellac layer, enabling the separation of PE materials from the paper substrate.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.889
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.222
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it