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Record W4309421754 · doi:10.21203/rs.3.rs-2163947/v1

Nanocores Magnetic Humic Acid on Montmorillonite Nanoneedles for Adsorption Dye Via RSM: Adsorption Isotherm, Kinetic Modelling and Thermodynamic Studies

2022· preprint· en· W4309421754 on OpenAlexaff
Zahra Abbasi, Abdolhadi Farrokhnia, Elisa I. García‐López, Zahra Zohrabzadeh, Ermia Aghaie, Yashar Behnamian

Bibliographic record

VenueResearch Square · 2022
Typepreprint
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsUniversity of AlbertaOkanagan University CollegeUniversity of British Columbia, Okanagan CampusUniversity of British Columbia
FundersShahid Chamran University of Ahvaz
KeywordsAdsorptionEndothermic processFreundlich equationGibbs free energyChemistryStandard molar entropyLangmuirEnthalpyAqueous solutionLangmuir adsorption modelMethyl orangeHumic acidStandard enthalpy of formationThermodynamicsPhysical chemistryOrganic chemistryPhotocatalysisCatalysis

Abstract

fetched live from OpenAlex

Abstract The current inquiry aimed at using core-shell Fe3O4@Humic acid/montmorillonite nanocomposites for removing methyl orange dye from an aqueous solution. The samples were characterized by FT-IR, TEM, SEM, XRD, BJH, and BET analytical methods. The efficiency removal has been utilized for 300 min reaction time using the response surface methodology by a design of five-factor-three-level central composite. The adsorption kinetics followed the pseudo-second-order rate kinetic model, showing an acceptable correlation (R2 > 0.99). Langmuir, Freundlich, Temkin, Dubinin–RadushKevich, and Harkins–Jura isotherms were utilized for the analysis of the equilibrium data. Also, we have estimated standard Gibbs free energy (∆G°), standard enthalpy (∆H°), standard entropy (∆S°), and the activation energy (Ea). The findings of this investigation suggest that the absorption of methyl orange on the adsorbent pursues the Frondelich isothermal formulation. The ∆G° values obtained showed physical absorption in this adsorption process. ∆H° showed that the dye adsorption mechanism was endothermic, and ∆S° indicated an increase in irregularity and the probability of contact between methyl orange molecules and the adsorbent surface in the dye adsorption process. Positive Ea values pointed out the nature of the endothermic absorption process. S* value was minimal and close to zero, which established the process of physical absorption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.068
GPT teacher head0.350
Teacher spread0.282 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2022
Admission routes1
Has abstractyes

Explore more

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