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Record W4310382841 · doi:10.26434/chemrxiv-2022-hxvcc

Augmenting Polymer Datasets by Iterative Rearrangement

2022· preprint· en· W4310382841 on OpenAlexafffund
Martin Seifrid, Théophile Gaudin, Alán Aspuru‐Guzik

Bibliographic record

VenueChemRxiv · 2022
Typepreprint
Languageen
FieldMaterials Science
TopicMachine Learning in Materials Science
Canadian institutionsVector InstituteCanadian Institute for Advanced ResearchUniversity of Toronto
FundersNatural Resources CanadaNational Research Council CanadaNatural Sciences and Engineering Research Council of Canada
KeywordsRepresentation (politics)Property (philosophy)Sequence (biology)EmbeddingComputer scienceArtificial intelligenceMachine learningChemistry

Abstract

fetched live from OpenAlex

One of the biggest obstacles to successful polymer property prediction is an effective representation that accurately captures the sequence of repeat units in a polymer. Motivated by the successes of data augmentation in computer vision and natural language processing, we explore augmenting polymer data by rearranging the molecular representation while preserving the correct connectivity, revealing additional substructural information that is not present in a single representation. We evaluate the effects of this technique on the performance of machine learning models trained on three experimental polymer datasets and compare them to common molecular representations. Data augmentation improves deep learning property prediction performance compared to equivalent (non-augmented) representations. In datasets where the target property is primarily influenced by the polymer sequence rather than experimental parameters, this data augmentation technique provides the molecular embedding with more information to improve property prediction accuracy.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.007
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.003
Threshold uncertainty score0.011

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.007
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0000.001
Scholarly communication0.0010.003
Open science0.0020.001
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0030.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.294
Teacher spread0.276 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2022
Admission routes2
Has abstractyes

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