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Record W4311021210 · doi:10.1038/s41598-022-24133-5

Microscopic revelation of the solid–gas coupling and Knudsen effect on the thermal conductivity of silica aerogel with inter-connected pores

2022· article· en· W4311021210 on OpenAlexafffund
Jing Liu, Piyapong Buahom, Chang Lu, Hou–Yong Yu, Chul B. Park

Bibliographic record

VenueScientific Reports · 2022
Typearticle
Languageen
FieldChemistry
TopicAerogels and thermal insulation
Canadian institutionsMcMaster UniversityUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of TorontoGovernment of Ontario
KeywordsAerogelThermal conductivityThermal conductionMaterials scienceThermodynamicsKnudsen numberConductivityCoupling (piping)ThermalComposite materialChemistryPhysical chemistryPhysics

Abstract

fetched live from OpenAlex

As a star insulation material, aerogel plays a significant role in saving energy and meeting temperature requirements in industry due to its extremely low thermal conductivity. The prediction of aerogel's thermal conductivity is of great interest in both research and industry, particularly because of the difficulty in measuring the separated gas conductivities directly by experiment. Hence, the proportions of separated gas conduction and solid-gas coupling conduction are debatable. In this work, molecular dynamics simulations were performed on porous silica aerogel systems to determine their thermal conductivities directly. The pore size achieved in the present study was improved significantly, making it possible to include the gas phase in the investigation of aerogel thermal conductivity. The separated solid conductivity [Formula: see text] and the separated gas thermal conductivity [Formula: see text] as well as the effective solid conductivity [Formula: see text] and the effective gas conductivity [Formula: see text] were calculated. The results suggest that the solid-gas coupling effect is negligible in rarefied gas because the enhancement of thermal conduction due to the short cut bridging effect by gas between gaps in the solid is limited. The gas pressure is the most significant factor that affects the solid-gas coupling effect. The large differential between the prediction and the actual value of the thermal conductivity is mainly from the underestimate of [Formula: see text], and not because of ignoring the coupling effect. As a conclusion, the solid-gas coupling effect can be neglected in the prediction of silica aerogel's thermal conductivity at low and moderate gas pressure, i.e., decreasing the gas pressure is the most efficient way to suppress the coupling effect. The findings could be used in multi-scale simulations and be beneficial for improving the accuracy of predictions of aerogel thermal conductivity.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.046
Threshold uncertainty score0.318

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.230
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2022
Admission routes2
Has abstractyes

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