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Simultaneous in situ Nitrate and Orthophosphate Measurement Using a Dual Chemistry Microfluidic Sensor

2022· article· en· W4312358520 on OpenAlexafffund
Edward Luy, James Smith, Iain Grundke, Colin Sonnichsen, Sean Morgan, Arnold Furlong, Vincent J. Sieben

Bibliographic record

VenueOCEANS 2022, Hampton Roads · 2022
Typearticle
Languageen
FieldChemical Engineering
TopicAnalytical Chemistry and Sensors
Canadian institutionsBedford Institute of OceanographyDartmouth General HospitalDalhousie University
FundersCanada First Research Excellence FundNational Research Council
KeywordsIn situMicrofluidicsNitrateDual (grammatical number)ChemistryEnvironmental chemistryNanotechnologyAnalytical Chemistry (journal)Materials scienceOrganic chemistry

Abstract

fetched live from OpenAlex

Anthropogenic nitrogen and phosphorus loading can have significant impact on land and marine based ecosystems with global impact. The use of nitrogen- and phosphorus-based fertilizers has continued to increase over recent years to stimulate agriculture production, and nutrient runoff from land can impact the stability of marine environments. As it stands, mitigation efforts are limited by a lack of comprehensive visibility over a wide spatial and temporal range, and severely impacted zones are often identified after significant ecological harm. Here, we present a submersible microfluidic sensor designed to simultaneously measure two prevalent forms of nitrogen and phosphorus, nitrate and orthophosphate, in situ within the same instrument. The device consists of two parallel analysis chambers, used to interrogate the same sample fluid with a different colourimetric assay for each species. To maintain small fluid volumes, light absorption spectrophotometry measurements are obtained using integral optical cells based on “inlaid microfluidics The performance of the dual-species nitrate and phosphate “NP Sensor” was first investigated in a controlled laboratory setting using prepared nutrient standards. A comprehensive temperature study followed to calibrate the sensor over a wide range of deployment conditions. Finally, the NP Sensor was deployed to acquire measurements in situ at two sites: a 60m vertical profile, and a long-term stationary shallow water study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.220
Teacher spread0.205 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2022
Admission routes2
Has abstractyes

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Same venueOCEANS 2022, Hampton RoadsSame topicAnalytical Chemistry and SensorsFrench-language works237,207