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Record W4313410376 · doi:10.1021/acssuschemeng.2c05233

Electrospinning of Softwood Organosolv Lignin without Polymer Addition

2022· article· en· W4313410376 on OpenAlexafffund
Maxime Parot, Denis Rodrigue, Tatjana Stevanovic

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2022
Typearticle
Languageen
FieldMaterials Science
TopicElectrospun Nanofibers in Biomedical Applications
Canadian institutionsUniversité Laval
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsOrganosolvSoftwoodLigninElectrospinningFiberPolymerMaterials scienceKraft paperChemical engineeringComposite materialChemistryPulp and paper industryOrganic chemistry

Abstract

fetched live from OpenAlex

Due to its nature and structure, lignin is a very difficult polymer to electrospin without any additives as only a few studies reported on the successful electrospinning of lignins in general and even more limited for softwood lignins to date. This paper highlights the possibility to use softwood organosolv lignin as a precursor for fiber electrospinning without any polymer addition. We have successfully electrospun pure organosolv softwood lignin into uniform, bead-free fibers. A concentration of 57 wt % of lignin in dimethyl formamide was determined as optimal, while other processing parameters (voltage, needle–collector distance, flow rate, and humidity) were studied to improve the fiber uniformity. We also studied the effects of minimum FeCl 3 addition and demonstrated its efficiency in improving the processability. Thus, the addition of 2 wt % FeCl 3 allowed decreasing the minimum fiber diameter from 400 to 200 nm. The addition of FeCl 3 also resolved the problem of fiber fusion on the collector, and it also allowed increasing the glass transition temperature of lignin fibers. These results open a way to new applications of lignin, such as 100% biosourced carbon fiber since no petroleum-sourced molecules were used in this study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.002
GPT teacher head0.185
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2022
Admission routes2
Has abstractyes

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