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Record W4316928142 · doi:10.1002/jeq2.20451

Mobility of arsenic and vanadium in waterlogged calcareous soils due to addition of zeolite and manganese oxide amendments

2023· article· en· W4316928142 on OpenAlexaff
Srimathie P. Indraratne, Chammi P. Attanayake, Darshani Kumaragamage, Geethani Amarawansha, Douglas M. Goltz, D. M. Applin

Bibliographic record

VenueJournal of Environmental Quality · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicArsenic contamination and mitigation
Canadian institutionsUniversity of Winnipeg
Fundersnot available
KeywordsSoil waterChemistryZeoliteAnoxic watersEnvironmental chemistryAlkalinityArsenicCalcareousManganeseAmendmentSoil pHAqueous solutionVanadiumInorganic chemistrySoil scienceGeology

Abstract

fetched live from OpenAlex

Abstract Addition of manganese(IV) oxides (MnO 2 ) and zeolite can affect the mobility of As and V in soils due to geochemical changes that have not been studied well in calcareous, flooded soils. This study evaluated the mobility of As and V in flooded soils surface‐amended with MnO 2 or zeolite. A simulated summer flooding study was conducted for 8 weeks using intact soil columns from four calcareous soils. Redox potential was measured in soils, whereas pH, major cations, and As and V concentrations were measured biweekly in pore water and floodwater. Aqueous As and V species were modeled at 0, 4, and 8 weeks after flooding (WAF) using Visual MINTEQ modeling software with input parameters of redox potential, temperature, pH, total alkalinity, and concentrations of major cations and anions. Aqueous As concentrations were below the critical thresholds (<100 μg L −1 ), whereas aqueous V concentrations exceeded the threshold for sensitive aquatic species (2–80 μg L −1 ). MnO 2 ‐amended soils were reduced to sub‐oxic levels, whereas zeolite‐amended and unamended soils were reduced to anoxic levels by 8 WAF. MnO 2 decreased As and V mobilities, whereas zeolite had no effect on As but increased V mobility, compared to unamended soils. Arsenic mobility increased under anoxic conditions, and V mobility increased under oxic and alkaline pH conditions. Conversion of As(V) to As(III) and V(V) to V(IV) was regulated by MnO 2 in flooded soils. MnO 2 can be used as an amendment in immobilizing As and V, whereas the use of zeolite in flooded calcareous soils should be done cautiously.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.783
Threshold uncertainty score0.351

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.261
Teacher spread0.248 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2023
Admission routes1
Has abstractyes

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