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Record W4317717856 · doi:10.1021/acs.cgd.2c01334

New Triclinic Polymorph of Tristearin

2023· article· en· W4317717856 on OpenAlexafffund
Saeed M. Ghazani, Alejandro G. Marangoni

Bibliographic record

VenueCrystal Growth & Design · 2023
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicFood Chemistry and Fat Analysis
Canadian institutionsUniversity of Guelph
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsTriclinic crystal systemCrystallographyChemistryLamellar structureCrystallizationMelting pointCrystal structureDiffractionOrganic chemistryOpticsPhysics

Abstract

fetched live from OpenAlex

Here we report on the discovery of a new triclinic crystal polymorphic form (β 1 ) of 1,2,3-stearoyl glycerol, or tristearin (SSS), CAS No. 555-43-1. This most stable polymorph of SSS has a melting point of 75.7 ± 0.5 °C and an enthalpy of fusion of 243.9 ± 10.5 J/g. The most stable polymorphic form for this well-known trisaturated monoacid triacylglycerol was obtained by static crystallization from a dilute solution of SSS in acetone at 4 °C over a period of 2 years. In contrast to the well-known β 2 form of tristearin, which displays wide-angle X-ray scattering reflection positions (relative intensities) at 4.61 Å (very strong), 3.86 Å (medium), and 3.70 Å (medium), the new β 1 tristearin displayed short-spacing positions (relative intensities) at 4.57 Å (weak), 3.84 Å (weak), and 3.68 Å (very strong). The small-angle X-ray scattering long-spacings corresponding to the lamellar sizes from the (001) plane were 44.91 Å, in contrast to 45.21 Å for the β 2 polymorph. This work clarifies controversies and uncertainties related to the number of triclinic polymorphs in trisaturated monoacid triaclyglycerols.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.080
Threshold uncertainty score0.794

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.044
GPT teacher head0.230
Teacher spread0.187 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2023
Admission routes2
Has abstractyes

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