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Record W4321501389 · doi:10.5194/egusphere-egu23-3609

Multi-method characterization of Asbestiform Antigorite from South Australia

2023· preprint· en· W4321501389 on OpenAlexaboutno aff
Alessandro Menini, Bao Han Truong, Seán Fitzgerald

Bibliographic record

Venuenot available
Typepreprint
Languageen
FieldMaterials Science
TopicClay minerals and soil interactions
Canadian institutionsnot available
Fundersnot available
KeywordsChrysotileMagentaTransmission electron microscopyPlatyMineralogyMineralChemistryCrystallographyMaterials sciencePolarizerComposite materialAsbestosMetallurgyNanotechnologyOptics

Abstract

fetched live from OpenAlex

Antigorite occurs in several locations worldwide and is defined as the simple serpentine Mg3Si205(OH)4 polymorph that compensates for the silica tetrahedral layer (Si2O5 sheet) misfit with the octahedral brucite Mg(OH)2 layer by regular structural undulation down the “b” crystalline axis. The chrysotile polymorph of the same chemistry compensates for the misfit in full rolls or scrolls along “b” axis, which can form fine fibres, and is the most common mineral in commercial asbestos. Chrysotile is therefore always asbestiform, but antigorite can exhibit a variety of crystalline habits in hand sample and the microscope, from massive, to platy, to bladed, and (occasionally) fibrous, but is not regulated as asbestos. Here, we performed a multi-method study in order to characterize a highly fibrous asbestiform occurrence of antigorite from Rowland Flat, South Australia. In comparison to HSE Canadian chrysotile, we show that optical (PLM) and transmission electron microscopy (TEM) allows to distinguish this antigorite from chrysotile. Based on PLM analysis with CS dispersion staining, chrysotile is magenta parallel (ǁ) to the polarizer and exhibits blue perpendicular (Ʇ) colours while this antigorite exhibits gold to golden magenta ǁ and blue-magenta Ʇ colours (1.550 HD RI at 25◦C). Also, we demonstrate SAED-TEM patterns for the two specimens to distinguish chrysotile “enrolled” crystal structure from the undulating antigorite structure, focusing on the highly characteristic [110] zone rel-rod streaking versus systematic repeats. Scanning electron microscopy (SEM) images were collected to further investigate the asbestiform nature of the antigorite from Rowland Flat. We show that the dominant morphology of Rowland Flat antigorite is of microscopic laths that split into very thin needles. In order to further investigate the morphometric parameters of this fibrous antigorite, individual fibres were measured at 20,000-25,000x by TEM. We show that the majority of these structures meet or exceed WHO fibres criteria, display high mean aspect ratios, ranging from 20:1 up to more than 100:1, and display widths lower than 1 µm, which in the literature is definition for asbestos fibres. Finally, our data indicate that the antigorite from Rowland Flat exhibits all characteristics of the asbestiform habit as defined in international standards (i.e., EPA/600/R-93/116), supporting the need for regulation of asbestiform antigorite as asbestos.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.020

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0020.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.149
GPT teacher head0.384
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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