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Record W4322756574 · doi:10.1016/j.fuel.2023.127864

Dynamics of soot surface growth and agglomeration by enclosed spray combustion of jet fuel

2023· article· en· W4322756574 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueFuel · 2023
Typearticle
Languageen
FieldChemical Engineering
TopicAdvanced Combustion Engine Technologies
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of CanadaEidgenössische Technische Hochschule ZürichSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungNational Science Foundation
KeywordsSootCombustionCrystalliteMaterials scienceAnalytical Chemistry (journal)Particle (ecology)Particle sizeJet (fluid)AerosolChemical engineeringMineralogyChemistryMetallurgyThermodynamicsEnvironmental chemistryOrganic chemistryPhysics

Abstract

fetched live from OpenAlex

Understanding the dynamics of soot formation and growth during combustion of jet fuel is essential for mitigation of aircraft engine emissions. Here, soot formation during enclosed spray combustion of jet fuel is investigated for its capacity to form soot with comparable characteristics to that from aircraft engines. For this, microscopy, scanning mobility particle, X-ray diffraction & Raman spectroscopy measurements and discrete element modeling (DEM) are employed along the flame centerline at various Effective eQuivalence Ratios (EQR). The DEM-derived mobility and primary particle size distribution dynamics are in excellent agreement with those measured at 5–63 cm height above the burner (HAB) for the measured temperature and soot volume fraction. At low EQR (1.46 and 1.59), soot surface growth stops at residence time, t = 4–7 ms, resulting in median soot primary particle diameters, d¯p, of ∼ 14 nm. At longer t (high HAB), agglomeration takes over increasing the median mobility diameter from 16 to 88 or 145 nm at EQR of 1.46 or 1.59, respectively, without altering d¯p and having the disorder over graphitic Raman band ratio, D/G = 0.9 ± 0.01 and a crystallite length, Lc = 1.24 ± 0.02 nm. In contrast, increasing EQR from 1.59 to 1.88, enhances soot surface growth, increases d¯p up to 23 nm and results in more graphitic soot having D/G = 0.8 ± 0.01 and Lc = 1.47 ± 0.01 nm. Furthermore, the D/G of soot is inversely proportional to its d¯p that is determined largely by surface growth.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.333
Threshold uncertainty score0.483

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.228
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it