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Record W4323821264 · doi:10.1002/9783527827992.ch48

The <scp>NORAM</scp> Process for the Production of Nitrobenzene (Case Study)

2023· other· en· W4323821264 on OpenAlexaff
Steven Buchi, Alfred Guenkel, Rob Pistner

Bibliographic record

Venuenot available
Typeother
Languageen
FieldMaterials Science
TopicThermal and Kinetic Analysis
Canadian institutionsNORAM (Canada)
Fundersnot available
KeywordsSulfuric acidNitrationChemistryNitric acidNitrobenzeneOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

The adiabatic nitration concept originated with American Cyanamid, who started up the first of two adiabatic mononitrobenzene (MNB) plants in the USA in 1979. At that time, the MNB production in the USA was 430 thousand MTPY and the global production was about one million MTPY. MNB is mostly converted to aniline, then to methylene diphenyl diisocyanate (MDI). In 1988, NORAM Engineering and Constructors was founded and developed a second-generation adiabatic MNB process. Since then, the global production of MNB has reached 12.5 million MTPY in 2020, with NORAM becoming the dominant technology provider with eighteen MNB plants in operation, accounting for over half of the global production. Four of the top five MDI producers operate multiple NORAM plants. In the NORAM MNB process, a large volume of sulfuric acid is circulated through the nitration loop to generate the reactive nitronium ion, to act as the dehydration agent, and to absorb the large heat of nitration without cooling. The sulfuric acid together with nitric acid and benzene are fed into the vertical plug flow nitrator, which uses high shear jet impingement mixing elements to generate interfacial area where the nitration reaction takes place. NORAM's plug flow nitrator inherently produces less byproducts than the continuously stirred tank reactors used in the original adiabatic process. The MNB and spent acid are separated by gravity, with the MNB continuing to product purification, and the spent acid being reconcentrated, and recycled to nitration, by flashing under vacuum. The crude MNB, containing stoichiometric excess benzene, nitrophenol byproducts, degradation products, and some other impurities, is purified to meet the MNB quality specifications. Effluents and vents are also treated to recover value products and to meet environmental standards. These unit operations account for the majority of the equipment in an MNB plant, and many of the decisions on which unit operations to implement are client and/or site specific. This chapter will discuss in detail the NORAM nitration process and present a review of various process steps and alternatives.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: Not applicable
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.634
Threshold uncertainty score0.390

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.287
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2023
Admission routes1
Has abstractyes

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