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Record W4327694676 · doi:10.1080/10601325.2022.2140674

Fabrication of poly(itaconic acid)-<i>g</i>-potassium alginate aerogels as eco-friendly biosorbents for removal of cationic dyes

2023· article· en· W4327694676 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Macromolecular Science Part A · 2023
Typearticle
Languageen
FieldChemistry
TopicAerogels and thermal insulation
Canadian institutionsUniversity of Alberta
FundersNational Natural Science Foundation of China
KeywordsAerogelCationic polymerizationAdsorptionMalachite greenChemistryMethylene blueNuclear chemistryItaconic acidFreundlich equationEnvironmentally friendlyChemical engineeringOrganic chemistryMaterials sciencePolymerNanotechnology

Abstract

fetched live from OpenAlex

Biosorbents derived from itaconic acid (IA) with abundant carboxyl groups are viewed as ideal materials for the removal of cationic dyes. However, it is still challenging to prepare IA-based biosorbents with satisfactory structural stability and adsorption ability. In this work, a novel poly(itaconic acid)-g-potassium alginate (PIA-g-PA) aerogel was prepared as a biosorbent and was then utilized to remove cationic dyes. The results presented that the as-prepared PIA-g-PA aerogel possessed outstanding adsorption capacities for cationic dyes based on the adsorption mechanism of electrostatic interaction. The adsorption process was well described by the pseudo-second-order model and the Freundlich model. The maximum adsorption capacities of the as-prepared aerogel toward methylene blue (MEB), malachite green (MG) and neutral red (NR) were 1892.07 mg·g−1, 786.96 mg·g−1 and 1169.23 mg·g−1, respectively. The adsorption capacity of aerogel toward cationic dyes significantly decreased with an increment of ionic strength. Meanwhile, the thermodynamic study indicated that the adsorption of cationic dyes onto the PIA-g-PA aerogel was spontaneous as an endothermic process. Additionally, the removal efficiency of as-prepared PIA-g-PA aerogel was still above 90.00% even after 10 cycles. Hence, the PIA-g-PA aerogel can be regarded as an eco-friendly adsorbent for the potential remediation of dye pollution in industrial effluents.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.498

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.288
Teacher spread0.272 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it