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Record W4362640547 · doi:10.2118/214684-pa

Apparent Heat of Reaction of Heavy Oil with Application of Accelerated Rate Calorimeter

2023· article· en· W4362640547 on OpenAlexaff
Rita Fazlyeva, D. G. Mallory, Gordon Moore, J. Modaresghazani, S. A. Mehta, Аlexey Cheremisin

Bibliographic record

VenueSPE Journal · 2023
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsOxygenChemistryCombustionCalorimeter (particle physics)Reaction rateThermodynamicsFlux (metallurgy)Analytical Chemistry (journal)CatalysisPhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Summary A series of accelerated rate calorimeter (ARC) experiments were conducted on heavy oil mixed with a carbonate core to study the thermal behavior and oxygen uptake operating at different air fluxes of 5.0, 2.5, and 1.25 (m3(ST)/(m2h)) referred to as Runs -1, -2 and -3, respectively. As a result, evaluation of the temperature rise per unit mass of oxygen was proposed as a new approach for identifying the main contributing mechanism during in-situ combustion (ISC). The obtained findings can be used for predicting the transition occurring between low- and high-temperature ranges (LTR and HTR). For Runs -2 and -3, such a transition occurred at 280°C, whereas for Run-1, operated at the highest air flux, LTR shifted to HTR at about 300°C. The overlapping curves of O2 to COx and O2 to low-temperature oxidation (LTO) plus water were interpreted as equal contributors to energy formation. The calculated maximum values varied between 4053 for LTO reactions and 13 420 dT(°C)dmO2(g) for high-temperature oxidation (HTO) reactions depending on the air flux. The measured self-heat rates (SHRs) and oxygen uptake, further used to obtain the apparent heat of reaction, were in general agreement with the values reported in the literature, 16 000 J/g O2 consumed. These values are typical for the HTO reactions; however, in this study, the heats of reaction when the oxidation reactions are operating in the oxygen addition or LTO mode were the main interest. Depending on the run, the apparent heats of LTO reactions varied between 4422 and 7101 J/g O2 consumed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.016
Threshold uncertainty score0.214

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.271
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2023
Admission routes1
Has abstractyes

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