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An inter-method comparison of mercury measurements in Icelandic volcanic gases

2023· article· en· W4362671234 on OpenAlexafffund
Brock A. Edwards, Melissa Pfeffer, Þorsteinn Jóhannsson, P.M. Outridge, Fei Wang

Bibliographic record

VenueApplied Geochemistry · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicMercury impact and mitigation studies
Canadian institutionsUniversity of ManitobaGeological Survey of CanadaNatural Resources Canada
FundersHáskóli ÍslandsNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsMercury (programming language)VolcanoPlumeEnvironmental scienceEnvironmental chemistryVolcanic GasesSampling (signal processing)Atmospheric sciencesChemistryMeteorologyGeologyGeochemistry

Abstract

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Volcanic systems are challenging environments in which to accurately sample or measure gaseous mercury (Hg) concentrations, as the gas plumes may be hot, acidic and halogen-rich; Hg concentrations may be highly variable; and the environment may not be readily accessible. We conducted an inter-method comparison study of atmospheric Hg measurements at Icelandic volcanic systems using four different methods. These included a passive air sampler (PAS), an active sampler with activated carbon trap (ACT) and two real-time measurement instruments, the Lumex portable mercury analyzer and the Tekran automated mercury analyzer. Good agreement in calculated and time-averaged volcanic plume Hg concentrations (ranging from 2.3 to 7.2 ng m−3) was obtained between the ACT and Lumex methods operated simultaneously at the same sites. In a post-fieldwork intercomparison, ACT and Tekran sampling yielded excellent agreement in measuring background atmospheric Hg concentrations. However, PAS-measured concentrations were significantly lower than the other methods, and in many cases were below the method detection limit, which may be due to the short sampling timeframes and/or adverse meteorological conditions not allowing sufficient Hg to be collected on the samplers. These findings demonstrate that Lumex and ACT methods are suitable for gaseous Hg measurement in volcanic gas plumes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.163
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.044
GPT teacher head0.340
Teacher spread0.296 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2023
Admission routes2
Has abstractyes

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