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Record W4362686088 · doi:10.1039/d3fd00065f

Effect of ionic conductivity of electrolyte on printed planar and vertical organic electrochemical transistors

2023· article· en· W4362686088 on OpenAlexafffund
Mona Azimi, Chi‐hyeong Kim, Jiaxin Fan, Fabio Cicoira

Bibliographic record

VenueFaraday Discussions · 2023
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsPolytechnique Montréal
FundersNatural Sciences and Engineering Research Council of CanadaDefence Research and Development CanadaCMC Microsystems
KeywordsTransconductanceElectrolyteMaterials scienceElectrochemistryTransistorIonic conductivityIonic bondingNanotechnologyConductivityIonic liquidPlanarIonMicrofabricationOptoelectronicsElectrodeChemistryComputer scienceElectrical engineeringVoltageOrganic chemistry

Abstract

fetched live from OpenAlex

Conducting polymers with mixed electronic/ionic transport are attracting a great deal of interest for applications in organic electrochemical transistors (OECTs). Ions play a crucial role in OECT performance. The concentration and mobility of ions in the electrolyte influence the current flow in the OECT and its transconductance. This study examines the electrochemical properties and ionic conductivity of two semi-solid electrolytes, iongels, and organogels, with diverse ionic species and properties. Our results indicate that the organogels exhibited higher ionic conductivities than the iongels. Furthermore, the geometry of OECTs plays an important role in determining their transconductance. Thus, this study employs a novel approach for fabricating vertical-configuration OECTs with significantly shorter channel lengths planar devices. This is achieved through a printing method that offers advantages, such as design versatility, scalability, expedited production time, and reduced cost relative to traditional microfabrication methods. The transconductance values obtained for the vertical OECTs were significantly (approximately 50 times) higher than those of the planar devices because of their shorter channel lengths. Finally, the impact of different gating media on the performance of both planar and vertical OECTs was studied, and devices gated by organogels demonstrated improved transconductance and switching speed (almost two times higher) than those gated by iongels.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.299

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.264
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2023
Admission routes2
Has abstractyes

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