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Record W4362717274 · doi:10.1016/j.supflu.2023.105941

Phase behavior of carbon dioxide + 2,4-dimethylpentane binary system at high pressures

2023· article· en· W4362717274 on OpenAlexfundno aff
Mihaela Ioniţă, Sergiu Sima, Adrian Victor Crişciu, Catinca Secuianu, Dan Vladimir Nichita

Bibliographic record

VenueThe Journal of Supercritical Fluids · 2023
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsnot available
FundersOntario Ministry of Research and InnovationUnitatea Executiva pentru Finantarea Invatamantului Superior, a Cercetarii, Dezvoltarii si InovariiCorporation for National and Community Service
KeywordsEquation of stateThermodynamicsvan der Waals forceIsothermal processBinary systemBar (unit)Mixing (physics)ChemistryBinary numberCarbon dioxideVapor–liquid equilibriumCubic functionOrganic chemistryPhysicsMeteorologyMolecule

Abstract

fetched live from OpenAlex

The phase behavior of the branched alkane 2,4-dimethyl pentane (2,4-DMP) and carbon dioxide (CO2) binary mixture that has no published data, to the best of our knowledge, was studied. The liquid–vapor critical line was determined up to 121.4 bar and 422.35 K, as well as vapor–liquid equilibrium (VLE) data at different constant temperatures (323.15, 343.15, 363.15, and 383.15) K and pressures between (10.4 and 120.4) bar. Phase behavior investigation was carried out in a high-pressures (HP) cell fitted with a pair of sapphire windows, one acting as a piston, hence volume up to 60 cm3, utilizing a static-analytical approach with phases sampling by the so called ROLSI valves (rapid online sample injectors) connected to a gas chromatograph (GC) for composition determination. The isothermal and critical data points for the carbon dioxide + 2,4-dimethylpentane binary mixture were modeled with the cubic equations of state (EoSs), i.e., Soave–Redlich–Kwong (SRK), Peng–Robinson (PR), and General Equation of State (GEOS), in combination with van der Waals mixing rules (one- and two-parameter conventional mixing rules, 1PCMR and 2PCMR). The calculations demonstrated that the selected models are capable of correctly reproducing the phase behavior of the mixture under study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.104
Threshold uncertainty score0.476

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.257
Teacher spread0.243 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2023
Admission routes1
Has abstractyes

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