Synergistic Tuning of CoO/CoP Heterojunction Nanowire Arrays as Efficient Bifunctional Catalysts for Alkaline Overall Water Splitting
Why this work is in the frame
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Bibliographic record
Abstract
Abstract Bifunctional electrocatalysts with superior activity and durability are of great importance for electrocatalytic water splitting. Herein, hierarchical structured CoO/CoP heterojunctions are successfully designed as highly efficient and freestanding bifunctional electrocatalysts toward overall water splitting. The unique microstructure combining two‐dimensional nanosheets with one‐dimensional nanowires enables numerous exposed active sites, shortened ion‐diffusion pathways, and enhanced conductivity, significantly improving performance. Such freestanding electrodes achieve high current density over 400 mA cm −2 at low overpotentials and have exceptional electrocatalytic activity as well as long‐term durability for both hydrogen and oxygen evolution reactions under alkaline conditions. Remarkably, a high current density of 20 mA cm −2 is generated at a low cell voltage of 1.56 V in an alkaline water electrolyzer, originating from synergistic interactions between CoO and CoP exposing active sites and facilitating charge transfer and enhancing kinetics. This work provides new insight into designing low‐cost but high‐performance bifunctional electrocatalysts for practical water splitting.
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Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.002 | 0.001 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.001 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.000 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it