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Record W4366181366 · doi:10.3390/separations10040261

Synthesis of Isoreticular Metal Organic Framework-3 (IRMOF-3) Porous Nanostructure and Its Effect on Naphthalene Adsorption: Optimized by Response Surface Methodology

2023· article· en· W4366181366 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueSeparations · 2023
Typearticle
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsUniversity of British Columbia, Okanagan CampusUniversity of British Columbia
FundersMinistry of Science and Technology, Taiwan
KeywordsNaphthaleneAdsorptionChemical engineeringPorosityWastewaterNanomaterialsNanostructureMaterials scienceMetal-organic frameworkSpecific surface areaChemistryInorganic chemistryNanotechnologyOrganic chemistryEnvironmental engineeringCatalysisEnvironmental science

Abstract

fetched live from OpenAlex

Naphthalene is a carcinogenic compound and its environmental release poses a major risk to human and aquatic health. Therefore, the application of nanomaterial technologies for naphthalene removal from wastewater has attracted significant attention. In this research, for the first time, the performance of IRMOF-3 for naphthalene removal from aqueous media is evaluated. IRMOF-3 with a specific surface area of 718.11 m2·g−1 has the ability to absorb naphthalene from synthetic wastewater to a high extent. The structures and morphology of IRMOF-3 were determined by FT-IR, XRD, SEM and BET analyses. Thirty adsorption experiments were conducted to obtain the best conditions for naphthalene removal. An optimum naphthalene removal efficiency of 80.96% was obtained at IRMOF-3 amounts of 0.1 g·L−1, a solution concentration of 15 mg·L−1, a contact time of 60 min and a pH = 11. The results indicate that the lower the concentration of naphthalene, the higher its dispersion at the surface of the porous nanostructure. Increasing naphthalene concentration results in its accumulation on porous nanostructures that clog cavities. In addition, high contact time provides ample opportunity for naphthalene to penetrate the cavities and pores which facilitates crystallization phenomena deep in the pores. Finally, the results of this study revealed that IRMOF-3 is one of the most effective adsorbents for naphthalene removal from wastewater.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.004
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.004
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.296
Teacher spread0.273 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it