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Record W4366486947 · doi:10.1021/acsomega.2c07812

New Approach to Shape Memory Polymer Composite Production Using Alkaline Lignin-Reinforced Epoxy-Based Shape Memory Polymers

2023· article· en· W4366486947 on OpenAlexafffund
Merve Uyan, Melih Soner Çeliktaş

Bibliographic record

VenueACS Omega · 2023
Typearticle
Languageen
FieldMaterials Science
TopicPolymer composites and self-healing
Canadian institutionsUniversity of Alberta
FundersTürkiye Bilimsel ve Teknolojik Araştırma KurumuEge ÜniversitesiUniversity of Alberta
KeywordsLigninDynamic mechanical analysisMaterials sciencePolymerFlexural strengthComposite materialModulusDifferential scanning calorimetryAlkaline hydrolysisShape-memory polymerEpoxyChemical engineeringChemistryOrganic chemistryHydrolysis

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide In the past few decades, there has been continued interest in shape memory polymers (SMPs), and tremendous efforts have been made to develop multifunctional composites of these SMPs to enhance the existing properties of SMPs. Although fossil-based sources are widely used in the production of shape memory polymer composites (SMPCs), the depletion of fossil-based resources and associated environmental problems increase interest toward renewable biobased products synthesized from natural resources. This study aims to produce alkaline lignin-reinforced SMPCs by using alkaline lignin in the SMP matrix. Thermo-mechanical, morphological, and shape memory tests are performed in order to reveal the effect of alkaline lignin usage in the SMP matrix on SMPC production. Differential scanning calorimetry analysis results show that adding alkaline lignin into the SMP matrix with 1 and 3% ratios led to an increase in T g values, while raising the alkaline lignin ratio to 5% decreased the T g value. According to the DMA results, increasing the alkaline lignin ratios caused an increase in the storage modulus of SMPCs, and the best storage modulus value was obtained at the 5% alkaline lignin ratio. The results of the three-point bending test also confirmed the results obtained from the DMA analysis, showing that an increasing alkaline lignin ratio caused an increase in the bending modulus. Scanning electron microscopy analysis showed a rough structure in 1 and 3% alkaline lignin supplementation, while a smoother structure was observed in 5% alkaline lignin supplementation. The smoother structure of the sample containing 5% alkaline lignin indicates that alkaline lignin supplementation exhibits a smoother surface by showing a plasticizing effect. As a result, it was observed that increasing the lignin ratio increased the polymer/alkaline lignin interaction, resulting in a harder structure and an increase in the flexural modulus value.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.092
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.002
Science and technology studies0.0010.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.034
GPT teacher head0.268
Teacher spread0.234 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2023
Admission routes2
Has abstractyes

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