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Record W4366751836 · doi:10.1016/j.coal.2023.104248

The occurrence of elevated δ34S in dissolved sulfate in a multi-level coal mine water system, Glasgow, UK

2023· article· en· W4366751836 on OpenAlexfundno aff
David B. Walls, Adrian J. Boyce, David Banks, Neil Burnside

Bibliographic record

VenueInternational Journal of Coal Geology · 2023
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsnot available
FundersNatural Environment Research CouncilSight Research UKUniversity of Guelph
Keywordsδ34SPyriteEvaporiteGeologySulfateGeochemistrySulfide mineralsSedimentary rockCarbonateGypsumMeteoric waterCarbonate mineralsAnhydriteCarboniferousSulfurCoal miningCoalCalciteChemistryPaleontologyFluid inclusionsHydrothermal circulation

Abstract

fetched live from OpenAlex

Stable isotopic compositions of δ18O, δ2H and dissolved sulfate δ34S in water from abandoned and flooded coal mines are used to interpret the water's and solutes' origin and interactive history. These isotopic ratios have been determined in mine water from a shallow (<100 m) series of overlapping coal mine workings at the UK Geoenergy Observatories Glasgow Geothermal Energy Research Field Site (UKGEOS GGERFS). Comparison has been made between dissolved sulfate δ34S of water in mined Carboniferous coal-bearing strata, that of water which had interacted with equivalent unmined strata, and δ34S in sulfide-bearing minerals (pyrite) in the host sedimentary rocks and local evaporite (gypsum) of the Lower Carboniferous Ballagan Formation. δ18O and δ2H confirm a meteoric origin for coal mine waters. The δ34S arithmetic mean and standard deviation of the pyrite (+5.0 ± 15.5‰) and water from unmined strata (+0.3 ± 2.1‰) were found to be similar, whereas the mine water exhibited elevated isotopic values (+20.3 ± 1.1‰), plotting closer to that of modern-day seawater (+21.2‰) and Ballagan Formation gypsum (+18.9 ± 0.5‰). Whilst the origin of dissolved sulfate in the mine water remains unclear, it is unlikely to be wholly due to simple pyrite oxidation. Influence of evaporite dissolution, fractionation associated with microbial sulfate reduction, and mixing with saline formation waters of marine, evaporitic or of another origin, cannot be ruled out.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.263

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.030
GPT teacher head0.262
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2023
Admission routes1
Has abstractyes

Explore more

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