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Record W4378983367 · doi:10.1016/j.seppur.2023.124237

Electric field-induced deformation and breakup of water droplets in polymer-flooding W/O emulsions: A simulation study

2023· article· en· W4378983367 on OpenAlex
Ning Li, Yunhui Pang, Zhiqian Sun, Yongxiang Sun, Zhuang Qi, Wangqing Li, Yue Liu, Bin Li, Zhenbo Wang, Hongbo Zeng

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueSeparation and Purification Technology · 2023
Typearticle
Languageen
FieldEngineering
TopicElectrohydrodynamics and Fluid Dynamics
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsNatural Science Foundation of Shandong ProvinceChina Scholarship CouncilMajor Scientific and Technological Innovation Project of Shandong ProvinceCanada Foundation for InnovationDepartment of Science and Technology of Shandong Province
KeywordsBreakupElectric fieldPolymerChemical physicsMaterials scienceMolecular dynamicsSteric effectsHydrogen bondMoleculeDeformation (meteorology)CounterionChemistryIonChemical engineeringComposite materialComputational chemistryMechanicsOrganic chemistryPhysics

Abstract

fetched live from OpenAlex

Polymers have a significant impact on the electrostatic demulsification efficiency of water-in-oil (W/O) emulsions by altering the motion characteristics of water droplets. To uncover the underlying micro-mechanism behind electric field-induced deformation and breakup of polymer-containing water droplets, we employed the molecular dynamics (MD) method to investigate the effect of different polymer concentrations ( c p ) on droplet motion under a DC electric field. The simulation results indicated that polyacrylamide (PAM) molecules possess a prominent electrostatic potential (ESP), resulting in a strong electrostatic attraction between PAM and water. The interface film of the droplet was found to exhibits high strength due to the formation of hydrogen bonds with a lifetime of 1 ps between polymers. The addition of polymers increased the polarity of the droplets, thereby promoting their deformation and breakup under an electric field. Both polarized polymers and ions migrated by carrying water molecules, which ultimately led to droplet breakup. At c p = 0.0221 mol·L −1 , the critical field strength ( E c ) for droplet breakup was the lowest, at only 0.672 V·nm −1 . As c p > 0.0221 mol·L −1 , the steric hindrance of PAM molecules and the strong interfacial film impeded the breakup of the droplets. These findings provided a theoretical basis for enhancing the electrostatic demulsification efficiency of polymer-flooding crude oil.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.899
Threshold uncertainty score0.333

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.258
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it