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Record W4381951267 · doi:10.1016/j.jcomc.2023.100376

A sustainable approach for developing biocarbon from lignin and its utilization in recycled ocean nylon based biocomposites

2023· article· en· W4381951267 on OpenAlexafffund
Zohrah B. Varsally, Neelima Tripathi, Haftom Weldekidan, Arturo Rodriguez‐Uribe, Oisik Das, Amar K. Mohanty, Manjusri Misra

Bibliographic record

VenueComposites Part C Open Access · 2023
Typearticle
Languageen
FieldEngineering
TopicLignin and Wood Chemistry
Canadian institutionsUniversity of Guelph
FundersOntario Agri-Food Innovation AllianceOntario Ministry of Economic Development, Job Creation and TradeMinistero dello Sviluppo EconomicoNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsMaterials scienceLigninFlexural strengthPyrolysisComposite materialFlexural modulusCelluloseFiller (materials)Nylon 6Pulp and paper industryPolymerChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Nylon/polyamide (PA6) is a major cause of ocean plastic pollution because of its extended use in commercial fishing activities. Recovery of this nylon from oceans and its use in manufacturing new materials or composites is urgently required to promote sustainability and circularity. In this work, unlike higher-density mineral fillers, lignin from the forestry industry was converted into biocarbon, which was used as a lightweight filler to manufacture recycled-ocean nylon (RN) based composites. Biocarbon is a highly stable, competitive, and sustainable filler for high-performance engineering plastics such as nylon. Lignin was pyrolyzed at 600°C followed by further treatment at 1200°C (with and without cobalt (II) nitrate catalyst) to induce graphitization in the produced biocarbon. Among the three types of biocarbon samples, such as pyrolyzed at 600°C, 1200°C and 1200°C catalyzed lignin biocarbon, the catalyzed biocarbon showed the maximum electrical conductivity. Catalyzed lignin biocarbon pyrolyzed at 1200°C showed an increase of 85% in electrical conductivity compared to commercial mineral graphite. The biocomposites consisting of 600°C biocarbon were manufactured by injection molding at different filler contents up to 40 wt.%. The biocomposites consisting of 40% of pyrolyzed lignin at 600°C showed increased flexural strength, flexural modulus, and heat deflection temperature by 41, 76 and 76%, respectively, compared to neat RN. Improved properties of the prepared biocarbons and biocomposites showed the potential of RN-based composites in the automotive industries.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.079
GPT teacher head0.336
Teacher spread0.257 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2023
Admission routes2
Has abstractyes

Explore more

Same venueComposites Part C Open AccessSame topicLignin and Wood ChemistryFrench-language works237,207