MétaCan
Menu
Back to cohort
Record W4382582136 · doi:10.1016/s1452-3981(23)15947-5

Synthesis, Crystal Structure, Spectral And Electrochemical Characterization, DNA Binding and Antioxidant studies of 1-(2- florobenzoyl)-3-(2-chloro, 4-ferrocenylphenyl) thiourea

2016· article· en· W4382582136 on OpenAlexfundno aff
Bhajan Lal, Sadia Akhter, Ataf Ali Altaf, Amin Badshah, Raja Azadar Hussain, Hui Li

Bibliographic record

VenueInternational Journal of Electrochemical Science · 2016
Typearticle
Languageen
FieldChemistry
TopicFerrocene Chemistry and Applications
Canadian institutionsnot available
FundersHEC MontréalHigher Education Commission, Pakistan
KeywordsChemistryCrystallographyBinding constantMoleculeMoietyThioureaAdductElectrochemistryCyclic voltammetryProton NMRSingle crystalDiffusionRing (chemistry)Crystal structureStereochemistryAnalytical Chemistry (journal)Physical chemistryBinding siteOrganic chemistryElectrode

Abstract

fetched live from OpenAlex

In this manuscript we have synthesized systematically 1-(2-florobenzoyl)-3-(2-chloro, 4-ferrocenylphenyl) thiourea (2F) and successfully determined the structure by single crystal X-rays diffraction analysis. The compound was spectrally characterized using multinuclear 1H and 13C nuclear magnetic resonance (NMR) and fourier transform infra-red (FT-IR) spectroscopic techniques and electrochemical characterization was carried out using cyclic voltammetry. The compound (2F) was then screened for potential deoxyribonucleic acid (DNA) binding and antioxidant activity. The single crystal XRD title compound 2F showed that ferrocenyl moiety had eclipsed conformation while the phenyl ring substituted on ferrocenyl is not in plane with cp-ring. The compound (2F) had shown a reversible process with one electron transfer, two peaks were observed for oxidation and reduction during scan. From voltametric measurements, the shifts in peak potential and peak current were used to review the mode of interaction which is found to be noncovalent electrostatic, drug-DNA binding constant and diffusion coefficients of the compound (2F) and 2F-DNA adduct. The binding constant (M-1) was found to be 2.92 × 103 with binding energy 19.76 kJ mol-1. The diffusion coefficient of free compound (2F) was calculated 1.75 × 10-7 whereas diffusion coefficient of 2F-DNA was found to less to i.e. 8.96 × 10-8 which was obvious as free molecules are easy to diffuse because of its low molecular weight whereas 2F interacted with DNA become heavier and the quantity of remained free molecules became less as a result decrease in current was observed. The compound (2F) showed significant activity with IC50 value 41.69 μg mL-1 using 1,1-diphenyl-2-picryl-hydrazyl (DPPH) assay.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.630

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.265
Teacher spread0.254 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2016
Admission routes1
Has abstractyes

Explore more

Same venueInternational Journal of Electrochemical ScienceSame topicFerrocene Chemistry and ApplicationsFrench-language works237,207