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Record W4384930695 · doi:10.1002/adfm.202305204

A Lean‐Zinc and Zincophilic Anode for Highly Reversible Zinc Metal Batteries

2023· article· en· W4384930695 on OpenAlex
Chao Li, Qingguo Shao, Kan Luo, Yiqiu Gao, Wenwen Zhao, Ning Cao, Shiyu Du, Xin Jin, Peichao Zou, Xiaobei Zang

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueAdvanced Functional Materials · 2023
Typearticle
Languageen
FieldEngineering
TopicAdvanced battery technologies research
Canadian institutionsMcGill University
FundersNatural Science Foundation of Shandong ProvinceState Key Laboratory of Heavy Oil ProcessingNational Natural Science Foundation of China
KeywordsAnodeZincMaterials scienceNucleationGalvanic anodeOverpotentialChemical engineeringMetalCobaltCathodeMetallurgyElectrodeCathodic protectionElectrochemistryChemistryPhysical chemistry

Abstract

fetched live from OpenAlex

Abstract Lean‐zinc anode is a promising configuration that can eliminate the trade‐off of energy density and cycle lifetime of zinc metal (Zn 0 ) batteries. However, there are rare investigations of lean‐Zn anode designs and it remains a grand change to sustain high zinc reversibility under lean zinc conditions. Herein, a lean‐Zn anode design based on a hierarchical and zincophilic cobalt metal (Co 0 ) nanowire‐decorated carbon host, which is derived from a ZnCo bimetallic organic framework, is reported. Within the lean‐Zn anode, the trace amount of Zn 0 acts as a zinc reservoir to make up for any irreversible loss of zinc source upon cycling, while the zincophilic Co 0 nanowires can guide uniform zinc nucleation and growth through a lattice matching mechanism. Consequently, high Zn 0 reversibility (average Coulomb efficiency of 99.6% for 4250 cycles), low nucleation overpotential (50.8 mV at 1 mA cm −2 ), and uniform and compact zinc electrodeposition are realized. When coupling the lean‐Zn anode with a Zn‐containing cathode, the full cell delivers high Coulomb efficiency (99.6% for 4250 cycles on average) and a long lifetime of more than 5000 cycles.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.052
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.259
Teacher spread0.234 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it